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We present experimental and theoretical studies of the absorption, emission and photodissociation spectra of Rb$_{2}$ molecules in solid helium. We have identified 11 absorption bands of Rb$_{2}$. All laser-excited molecular states are…

Atomic Physics · Physics 2009-11-11 P. Moroshkin , A. Hofer , S. Ulzega , A. weis

The optical absorption spectrum of the three most stable isomers of the Ag11 system was calculated using the time-dependent density functional theory, with the generalized gradient approximation for the exchange and correlation potential,…

Atomic and Molecular Clusters · Physics 2009-11-13 Jose I. Martinez , Eva M. Fernandez

The ultrafast response of the prototype Mott-Hubbard system (V1-xCrx)2O3 was systematically studied with fs pump-probe reflectivity, allowing us to clearly identify the effects of the metal-insulator transition on the transient response.…

Strongly Correlated Electrons · Physics 2011-08-29 B. Mansart , D. Boschetto , S. Sauvage , A. Rousse , M. Marsi

Photoabsorption of atomic oxygen in the energy region below the $\rm 1s^{-1}$ threshold in x-ray spectroscopy from {\it Chandra} and {\it XMM-Newton} is observed in a variety of x-ray binary spectra. Photoabsorption cross sections…

High Energy Astrophysical Phenomena · Physics 2015-06-16 B. M. McLaughlin , C. P. Ballance , K. P. Bowen , D. J. Gardenghi , W. C. Stolte

Attosecond light pulses in the extreme ultraviolet have drawn a great deal of attention due to their ability to interrogate electronic dynamics in real time. Nevertheless, to follow charge dynamics and excitations in materials, element…

Atomic Physics · Physics 2016-06-08 S. M. Teichmann , F. Silva , S. L. Cousin , M. Hemmer , J. Biegert

Nonlinear THz-THz-Raman (TTR) liquid spectroscopy offers new possibilities for studying and understanding condensed-phase chemical dynamics. Although TTR spectra carry rich information about the systems under study, the response is encoded…

Chemical Physics · Physics 2019-08-20 Ioan B. Magdau , Griffin J. Mead , Geoffrey A. Blake , Thomas F. Miller

We present new evidence of X-ray absorption variability on time scales from a few hours to a few days for several nearby bright AGNs. The observed N_H variations imply that the X-ray absorber is made of clouds eclipsing the X-ray source…

Cosmology and Nongalactic Astrophysics · Physics 2015-05-14 Guido Risaliti

We present a model of coherent Bremsstrahlung emission from the compression phase of relativistic heavy ion collisions based on a hydrodynamical description of the collision process. The decceleration of the matter through a shock front,…

High Energy Physics - Phenomenology · Physics 2007-05-23 C. Bertulani , L. Mornas , U. Ornik

Charge transport processes at interfaces which are governed by complex interfacial electronic structure play a crucial role in catalytic reactions, energy storage, photovoltaics, and many biological processes. Here, the first soft X-ray…

The photon energy spectrum in inclusive weak radiative B -> X_s gamma decay is computed to order alpha_s^2 beta_0. This result is used to extract a value for the HQET parameter $\bar\Lambda$ from the average <1-2E_\gamma/m_B>, and a value…

High Energy Physics - Phenomenology · Physics 2011-05-05 Zoltan Ligeti , Michael Luke , Aneesh V. Manohar , Mark B. Wise

High-harmonic spectroscopy (HHS) in liquids promises real-time access to ultrafast electronic dynamics in the native environment of chemical and biological processes. While electron recollision has been established as the dominant mechanism…

We theoretically investigate the role of complex dipole phase in the attosecond probing of charge migration. The iodobromoacetylene ion (ICCBr$^+$) is considered as an example, in which one can probe charge migration by accessing both the…

Chemical Physics · Physics 2022-02-23 Yuki Kobayashi , Daniel M. Neumark , Stephen R. Leone

We use a simple generic model to study the desorption of atoms from a solid surface in contact with a liquid, by using a combination of Monte Carlo and molecular dynamics simulations. The behavior of the system depends on two parameters:…

Chemical Physics · Physics 2022-11-16 Krishna Jaiswal , Horia Metiu , Vishal Agarwal

Time-dependent density functional theory (TDDFT) has been applied to the calculation of absorption spectra for two-dimensional atomic layer materials. We reveal that the character of the first bright exciton state of bi-layer hexagonal…

Materials Science · Physics 2020-01-08 Yasumitsu Suzuki , Kazuyuki Watanabe

Highly excited states of rubidium (Rb) atoms attached to helium (He) nanodroplets are studied by two-photon ionization spectroscopy in combination with electron and ion imaging. Photoion spectra and angular distributions are in good…

Atomic and Molecular Clusters · Physics 2017-08-23 L. Fechner , B. Gruener , A. Sieg , C. Callegari , F. Ancilotto , F. Stienkemeier , M. Mudrich

Transient grating acoustic spectroscopy has been applied to studies on the vibrational energy relaxation process of the electronic ground state of azulene, two 1-alkylazulenes, and five bridged azulene-anthracenes in three different…

Materials Science · Physics 2014-06-18 Hiroki Fujiwara

In semiconductors, the identification of doping atomic elements allowing to encode a qubit within spin states is of intense interest for quantum technologies. In transition metal dichalcogenides semiconductors, the strong spin-orbit…

Broadband ultrafast optical spectroscopy methods, such as transient absorption spectroscopy and 2D spectroscopy, are widely used to study molecular dynamics. However, these techniques are typically restricted to optically thick samples,…

Optics · Physics 2021-04-29 Myles C. Silfies , Grzegorz Kowzan , Neomi Lewis , Thomas K. Allison

Modelling of thermonuclear X-ray bursts on accreting neutron stars has to date focused on stable accretion rates. However, bursts are also observed during episodes of transient accretion. During such events, the accretion rate can evolve…

High Energy Astrophysical Phenomena · Physics 2018-03-28 Zac Johnston , Alexander Heger , Duncan K. Galloway

We have detected transient X-ray activity from the X-ray burster 4U~0614+091 simultaneously with BATSE/CGRO (20-100 keV) and ASM/RXTE (1-12 keV). The peak fluxes reach approximately 40 mCrab in both instruments over a period of about 20…

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