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Temporal evolution of transient absorption spectra for pre-solvated electron (e-) generated by biphotonic (200 nm) ionization of liquid H2O and D2O has been studied on femto- and pico- second time scales. These spectra were obtained in the…

Chemical Physics · Physics 2007-05-23 Rui Lian , Robert A. Crowell , Ilya A. Shkrob

We extend the first-principles analysis of attosecond transient absorption spectroscopy to two-dimensional materials. As an example of two-dimensional materials, we apply the analysis to monolayer hexagonal boron nitride (h-BN) and compute…

Materials Science · Physics 2019-07-19 Shunsuke A. Sato , Hannes Hübener , Umberto De Giovannini , Angel Rubio

Time integrated spectroscopic measurements are carried out to characterize transient plasma stream produced in a coaxial pulsed plasma accelerator. This method allows the estimation of different plasma parameters and its evolution with…

Plasma Physics · Physics 2020-08-04 A. Ahmed , S. Singha , S. Borthakur , N. K. Neog , T. K. Borthakur , J. Ghosh

Dielectric loss spectra covering 13 decades in frequency were collected for 2-ethyl-1-hexanol, a monohydroxy alcohol that exhibits a prominent Debye-like relaxation, typical for several classes of hydrogen-bonded liquids. The thermal…

Soft Condensed Matter · Physics 2012-03-12 C. Gainaru , S. Kastner , F. Mayr , P. Lunkenheimer , S. Schildmann , H. J. Weber , W. Hiller , A. Loidl , R. Böhmer

We report the discovery of a transient equivalent hydrogen column density with an absorption edge at ~3.8 kiloelectron volts in the spectrum of the prompt x-ray emission of gamma-ray burst (GRB) 990705. This feature can be satisfactorily…

We calculate the transient absorption of an isolated attosecond pulse by helium atoms subject to a delayed infrared (\ir) laser pulse. With the central frequency of the broad attosecond spectrum near the ionization threshold, the absorption…

Atomic Physics · Physics 2015-06-12 Shaohao Chen , Mengxi Wu , Mette B. Gaarde , Kenneth J. Schafer

Photo-stimulated desorption (PSD) of Xe atoms from the Au(001) surface in thermal and nonthermal regimes was investigated by the time-of-flight measurement at photon energies of 6.4 and 2.3 eV. Xe was desorbed in a thermal way at high laser…

Mesoscale and Nanoscale Physics · Physics 2016-06-14 Akihiko Ikeda , Masuaki Matsumoto , Shohei Ogura , Katsuyuki Fukutani , Tatsuo Okano

Time-resolved X-ray absorption spectroscopy has been utilized to monitor the bimolecular electron transfer in a photocatalytic water splitting system for the first time. This has been possible by uniting the local probe and element specific…

We investigate the characteristic effects of nuclear motion on attosecond transient absorption spectra in molecules by calculating the spectrum for different model systems. Two models of the hydrogen molecular ion are considered: one where…

Atomic Physics · Physics 2015-04-16 Jens E. Bækhøj , Lun Yue , Lars Bojer Madsen

Both single-laser and two-laser experiments were conducted to look into the ion-imaging of Br*(2P1/2) and Br(2P3/2) photo-fragmented from 1-bromo-2-methylbutane in the range 232-240 nm via a detection scheme of (2+1) resonance-enhanced…

The electronic excitation occurring on adsorbates at ultrafast time scales from optical lasers that initiate surface chemical reactions is still an open question. Here, we report the ultrafast temporal evolution of X-ray absorption…

We investigate the possibility to use transient absorption of a coherent bound electron wave packet in hydrogen as an attosecond pulse characterization technique. In recent work we have shown that photoionization of such a coherent bound…

Optics · Physics 2017-11-22 Jan Marcus Dahlström , Stefan Pabst , Eva Lindroth

X-ray spectroscopy has been a key method to determine ground and excited state properties of quantum materials with atomic specificity. Now, new x-ray facilities are opening the door to the study of pump-probe x-ray spectroscopy -…

Strongly Correlated Electrons · Physics 2025-02-11 Daniel Jost , Eder G. Lomeli , Ta Tang , Joshua J. Kas , John J. Rehr , Wei-Sheng Lee , Hong-Chen Jiang , Brian Moritz , Thomas P. Devereaux

A number of emission and absorption features are expected to be visible in high energy resolution X-ray spectra of type 1 AGN with ionized gas along the line of sight (so called "warm absorbers"). Emission strongly depends on the…

Astrophysics · Physics 2007-05-23 F. Nicastro , F. Fiore , G. Matt

The x-ray absorption spectra of water and ice are calculated with a many-body approach for electron-hole excitations. The experimental features, including the small effects of temperature change in the liquid, are quantitatively reproduced…

Soft Condensed Matter · Physics 2015-05-14 Wei Chen , Xifan Wu , Roberto Car

High-resolution spectroscopy allows one to probe weak interactions and to detect subtle phenomena. While such measurements are routinely performed on atoms and molecules in the gas phase, spectroscopy of adsorbed species on surfaces is…

X-ray absorption spectroscopy was used to study the microscopic origin of conductance and resistive switching in chromium doped strontium titanate (Cr:SrTiO3). Differences in the x-ray absorption near edge spectroscopy (XANES) at the Cr…

Materials Science · Physics 2007-07-05 B. P. Andreasson , M. Janousch , U. Staub , G. I. Meijer , B. Delley

We present a time-resolved spectrophotometric study of the optical variability in the quiescent soft X-ray transient A0620-00. Superimposed on the double-humped continuum lightcurve are the well known flare events which last tens of…

Absorption spectra of liquid water at 300 K are calculated from both classical and density functional theory molecular dynamics simulation data, which together span from 1 MHz to hundreds of THz, agreeing well with experimental data…

Chemical Physics · Physics 2020-09-09 Shane Carlson , Florian N. Brünig , Philip Loche , Douwe Jan Bonthuis , Roland R. Netz

It is possible that the proton is stable while atomic hydrogen is not. This is the case in models with new particles carrying baryon number which are light enough to be stable themselves but heavy enough so that proton decay is…

High Energy Physics - Phenomenology · Physics 2020-03-06 David McKeen , Maxim Pospelov
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