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Related papers: Atomic oxygen adsorption and incipient oxidation o…

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By means of density functional theory we have undertaken a structural, electronic and magnetic survey of the adsorption of the Fe_xPt_y(x,y=<4) clusters on MgO (001) surface under the generalized gradient approximation. We have tested…

Materials Science · Physics 2015-06-23 Ramon Cuadrado , Roy W. Chantrell

Ab initio total energy calculations within the framework of density functional theory have been performed for atomic hydrogen and oxygen chemisorption on the (0001) surface of double hexagonal packed americium using a full-potential…

Strongly Correlated Electrons · Physics 2015-05-14 P. P. Dholabhai , R. Atta-Fynn , A. K. Ray

We present a detailed study of the adsorption of CO on Cu, Rh, and Pt (111) surfaces in top and hollow sites. The study has been performed using the local density approximation, the gradient corrected functional PBE, and the hybrid…

Materials Science · Physics 2011-12-30 A. Stroppa , K. Termentzidis , J. Paier , G. Kresse , J. Hafner

Large scale first-principles calculations based on density functional theory (DFT) employing two different methods (atomic orbitals and plane wave basis sets) were used to study the energetics, geometry, the electronic charge redistribution…

Materials Science · Physics 2010-05-27 Vitaly Alexandrov , Sergei Piskunov , Yuri F. Zhukovskii , Eugene A. Kotomin , Joachim Maier

Extensive density-functional calculations are performed for chemisorption of atoms in the three first periods (H, B, C, N, O, F, Al, Si, P, S, and Cl) on the polar TiC(111) surface. Calculations are also performed for O on TiC(001), for…

Materials Science · Physics 2007-05-23 Carlo Ruberto , Bengt I. Lundqvist

We report static and dynamic first-principles calculations that provide atomistic pictures of the initial stage of the oxidation processes occurring at the ($11\bar20$) surface of 4H-SiC. Our results unveil reaction pathways and their…

Materials Science · Physics 2017-02-15 Han Li , Yu-ichiro Matsushita , Mauro Boero , Atsushi Oshiyama

We investigate the adsorption of cobalt phthalocyanine (CoPc) molecules on a thin layer of cobalt oxide grown on Ir(100). To that end we compare the results of low-temperature scanning tunneling microscopy (STM) with those of ab-initio…

Mesoscale and Nanoscale Physics · Physics 2018-10-24 Tobias Schmitt , Pascal Ferstl , Lutz Hammer , M. Alexander Schneider , Josef Redinger

Results of recent density functional theory calculations for alkali metal adsorbates on close-packed metal surfaces are discussed. Single adatoms on the (111) surface of Al and Cu are studied with the self-consistent surface Green-function…

mtrl-th · Physics 2016-09-07 C. Stampfl , M. Scheffler

The adsorption and dissociation of O$_{2}$ molecules at the Be(0001) surface is studied by using density-functional theory within the generalized gradient approximation and a supercell approach. The physi- and chemisorbed molecular…

Materials Science · Physics 2013-05-29 Ping Zhang , Bo Sun , Yu Yang

The structures and energetics of organic molecules adsorbed onto clean and H-passivated Si(001)-(2$\times$1) surfaces have been calculated using density functional theory. For benzene adsorbed on the clean Si surface the tight-bridge…

Materials Science · Physics 2009-11-13 Karen Johnston , Risto M. Nieminen

Oxygen adsorption onto Ru (10 bar 1 0) results in the formation of two ordered overlayers, i.e. a c(2 times 4)-2O and a (2 times 1)pg-2O phase, which were analyzed by low-energy electron diffraction (LEED) and density functional theory…

We present and discuss the results of ab initio DFT plane-wave supercell calculations of the atomic and molecular oxygen adsorption and diffusion on the LaMnO3 (001) surface which serves as a model material for a cathode of solid oxide fuel…

Materials Science · Physics 2008-02-04 Eugene A. Kotomin , Yuri A. Mastrikov , Eugene Heifets , Joachim Maier

The results of DFT supercell calculations of oxygen behavior upon the UN (001) and (110) surfaces as well as at the tilt grain boundary are presented. Oxygen adsorption, migration, incorporation into the surface N vacancies on (001) and…

Materials Science · Physics 2015-06-12 D. Bocharov , D. Gryaznov , Yu. F. Zhukovskii , E. A. Kotomin

Ab initio self-consistent total energy calculations using second order Moller-Plesset perturbation theory and Hay-Wadt effective core potentials for gallium and arsenic have been used to investigate the chemisorption of atomic oxygen on the…

Condensed Matter · Physics 2007-05-23 Michael L. Mayo , Asok K. Ray

A series of First Principles calculations is undertaken to characterize and explain the enhancement of the catalytic activity of oxygen on top of very disordered nanomaterials of Pt. As the adsorption of OH fragment on top of the surfaces…

Materials Science · Physics 2024-02-02 Olivier Le Bacq

We present a systematic analysis of molecular oxygen (O$_2$) adsorption trends on bimetallic PtNi clusters and their monometallic counterparts supported on MgO(100), by means of periodic DFT calculations for sizes between 25 up to 58 atoms.…

Materials Science · Physics 2016-04-12 Lauro Oliver Paz-Borbon , Francesca Baletto

Indium oxide offers optical transparency paired with electric conductivity, a combination required in many optoelectronic applications. The most-stable In2O3(111) surface has a large unit cell (1.43 nm lattice constant). It contains a…

Fabrication, handling and disposal of nuclear fuel materials require comprehensive knowledge of their surface morphology and reactivity. Due to unavoidable contact with air components (even at low partial pressures), UN samples contain…

Materials Science · Physics 2010-09-01 Yuri F. Zhukovskii , Dmitry Bocharov , Eugene Kotomin , Robert Evarestov , Andrey V. Bandura

Atom controlled sub-nanometer MoS$_2$ pores have been recently fabricated. Oxidative environments are of particular interest for MoS$_2$ applications in electronics, sensing and energy storage. In this work we carried out first-principles…

Materials Science · Physics 2023-01-31 Murilo Kendjy Onita , Flavio Bento de Oliveira , Andreia Luisa da Rosa

Density-functional calculations on the polar TiX(111) (X = C, N) surfaces show (i) for clean surfaces, strong Ti3d-derived surface resonances (SR's) at the Fermi level and X2p-derived SR's deep in the upper valence band and (ii) for adatoms…

Materials Science · Physics 2009-11-11 Carlo Ruberto , Aleksandra Vojvodic , Bengt I. Lundqvist