Related papers: Enhancing single-molecule photostability by optica…
Single dye molecules at cryogenic temperatures display many spectroscopic phenomena known from free atoms and are thus promising candidates for fundamental quantum optical studies. However, the existing techniques for the detection of…
We propose a technique to improve the probability of single-photon emission with an electrically pumped quantum dot in an optical microcavity, by continuously monitoring the energy state of the dot and using feedback to control when to stop…
The quantum-jump approach is used for a theoretical description of resonance luminescence from a {\em single} semiconductor quantum dot in contact with its solid-state environment. For continuous excitation of the single-exciton groundstate…
Producing advanced quantum states of light is a priority in quantum information technologies. While remarkable progress has been made on single photons and photon pairs, multipartite correlated photon states are usually produced in purely…
A holy grail of photonics research is the realization of a laser that uses a single quantum emitter as the gain medium. Such a device would exhibit a plethora of new features, including lasing without a well-defined threshold and output…
An engineering technique using continuous quantum measurement together with a change detection algorithm is proposed to improve the probability of single photon emission for a quantum-dot based single-photon source. The technique involves…
Triggered single-photon sources produce the vacuum state with non-negligible probability, but produce a much smaller multiphoton component. It is therefore reasonable to approximate the output of these photon sources as a mixture of the…
Quantum technologies, holding the promise of exponentially superior performance than their classical counterparts for certain tasks, have consistently encountered challenges, including instability in quantum light sources, quantum…
Single photon detectors have historically consisted of macroscopic-sized materials but recent experimental and theoretical progress suggests new approaches based on nanoscale and molecular electronics. Here we present a theoretical study of…
The ability to efficiently produce and manipulate nonclassical states of light is a critical requirement for the development of quantum optical technologies. In recent years, experiments have demonstrated that cascaded spontaneous…
Single photon detection generally consists of several stages: the photon has to interact with one or more charged particles, its excitation energy will be converted into other forms of energy, and amplification to a macroscopic signal must…
Radiative decay from the excited $^1P_1$ state to metastable $^3P_2$ and $^3P_0$ states is expected to limit attainable trapped atomic population in a magneto-optic trap of ytterbium (Yb) atoms. In experiments we have carried out with…
It depends. For a single molecule interacting with one mode of a biphoton probe, we show that the spectroscopic information has three contributions, only one of which is a genuine two-photon contribution. When all the scattered light can be…
Discharge and electron-impact excitation lead to the production of metastable helium atoms in two metastable states, 2$^1$S$_0$ and 2$^3$S$_1$. However, many applications require pure beams of one of these species or at least a detailed…
There has been considerable progress in electro-statically emptying, and re-filling, quantum dots with individual electrons. Typically the quantum dot is defined by electrostatic gates on a GaAs/AlGaAs modulation doped heterostructure. We…
We show that it is possible to ``store'' quantum states of single-photon fields by mapping them onto {\it collective} meta-stable states of an optically dense, coherently driven medium inside an optical resonator. An adiabatic technique is…
The photoinduced excited-state dynamics of the keto and enol forms of cytosine is investigated using ab initio surface hopping in order to understand the outcome of molecular beam femtosecond pump-probe photoionization spectroscopy…
By employing single charge injections with an atomic force microscope, we investigated redox reactions of a molecule on a multilayer insulating film. First, we charged the molecule positively by attaching a single hole. Then we neutralized…
A scanning tunneling microscope (STM) can do more than atomic imaging and manipulation. Its tunneling current can also be used for the excitation of light, converting electron energy to photon energy. STM based single-molecule…
We demonstrate by time-resolved resonance fluorescence measurements on a single self-assembled quantum dot an internal photo-effect that emits electrons from the dot by an intra-band excitation. We find a linear dependence of the optically…