Related papers: Enhancing single-molecule photostability by optica…
The coherent interaction of electromagnetic fields with solid-state two-level systems can yield deterministic quantum light sources for photonic quantum technologies. To date, the performance of semiconductor single-photon sources based on…
The high quantum efficiency of photosynthetic complexes has inspired researchers to explore new routes to utilize this process for photovoltaic devices. Quantum coherence has been demonstrated to play a crucial role within this process.…
We propose a scheme to transfer molecules from a slow beam into an optical trap using only a single photon absorption and emission cycle. The efficiency of such a scheme is numerically explored for BaF using realistic experimental…
We investigate the dynamical process of optically trapped X$^{1}$$\Sigma$$^{+}$ (v" = 0) state $^{85}$Rb$^{133}$Cs molecules distributing in J" = 1 and J" = 3 rotational states. The considered molecules, formed from short-range…
Understanding molecular state evolution is central to many disciplines, including molecular dynamics, precision measurement, and molecule-based quantum technology. Details of the evolution are obscured when observing a statistical ensemble…
We demonstrate the conversion of cold Cs_{2} molecules initially distributed over several vibrational levels of the lowest triplet state a^{3}\Sigma_{u}^{+} into the singlet ground state X^{1}\Sigma_{g}^{+}. This conversion is realized by a…
An explanation is provided for the ultrafast photo-excited electron dynamics in low-spin Ruthenium (II) organic complexes. The experimentally-observed singlet to triplet decay in the metal-to-ligand charge-transfer (MLCT) states contradicts…
The generation of single photons using solid-state quantum emitters is pivotal for advancing photonic quantum technologies, particularly in quantum communication. As the field continuously advances towards practical use cases and beyond…
Current single-molecule imaging techniques are incapable of providing stochastic information of individual chemical reactions. We have developed an optical imaging method for stochastic analysis of individual electrochemical reactions. The…
We report significant improvements in the retrieval efficiency of a single excitation stored in an atomic ensemble and in the subsequent generation of strongly correlated pairs of photons. A 50% probability to transform the stored…
We investigate a singly-charged quantum dot under a strong optical driving field by probing the system with a weak optical field. When the driving field is detuned from the trion transition, the probe absorption spectrum is shifted from the…
Path-entangled multi-photon states allow optical phase-sensing beyond the shot-noise limit, provided that an efficient parity measurement can be implemented. Realising this experimentally is technologically demanding, as it requires…
We demonstrate two solid-state sources of indistinguishable single photons. High resolution laser spectroscopy and optical microscopy were combined at T = 1.4 K to identify individual molecules in two independent microscopes. The Stark…
Analogous to Coulomb blockade for electrons, photon blockade is a key quantum optical effect in which the presence of one photon prevents the transmission of subsequent ones through a nonlinear medium. Beyond its fundamental interest,…
Photon upconverters are anti Stokes emitters capable of generating photons with higher energy than those absorbed. This behavior can be achieved through different mechanisms, which are extensively studied for applications in imaging,…
Singlet fission may boost photovoltaic efficiency [by transforming a singlet exciton into two triplet excitons and thereby doubling the number of excited charge carriers. The primary step of singlet fission is the ultrafast creation of the…
A scheme for exploring photon number amplification and discrimination is presented based on the interaction of a large number of two-level atoms with a single mode radiation field. The fact that the total number of photons and atoms in the…
The long spin coherence times in ambient conditions of color centers in solids, such as nitrogen-vacancy (NV$^{-}$) centers in diamond, make these systems attractive candidates for quantum sensing. Quantum sensing provides remarkable…
The energy states in semiconductor quantum dots are discrete as in atoms, and quantum states can be coherently controlled with resonant laser pulses. Long coherence times allow the observation of Rabi-flopping of a single dipole transition…
In practice, single photons are generated as a mixture of vacuum with a single photon with weights 1-p and p, respectively; here we are concerned with increasing p by directing multiple copies of the single photon-vacuum mixture into a…