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We present a versatile density functional approach (DFT) for calculating the depletion potential in general fluid mixtures. In contrast to brute force DFT, our approach requires only the equilibrium density profile of the small particles…

Soft Condensed Matter · Physics 2009-10-31 R. Roth , R. Evans , S. Dietrich

A mesoscopic theory for the primitive model of ionic systems is developed for arbitrary size, $\lambda=\sigma_+/\sigma_-$, and charge, $Z=e_+/|e_-|$, asymmetry. Our theory is an extension of the theory we developed earlier for the…

Statistical Mechanics · Physics 2009-11-10 A. Ciach , W. T. Góźdź , G. Stell

The recent generalized Debye-Hueckel (GDH) theory is applied to the calculation of the charge-charge correlation function G_{ZZ}(r). The resulting expression satisfies both (i) the charge neutrality condition and (ii) the Stillinger-Lovett…

Statistical Mechanics · Physics 2008-02-03 Benjamin P. Lee , Michael E. Fisher

The kinetic theory description of a low density gas of hard spheres or disks, confined between two parallel plates separated a distance smaller than twice the diameter of the particles, is addressed starting from the Liouville equation of…

Statistical Mechanics · Physics 2024-09-06 J. Javier Brey , M. I. García de Soria , P. Maynar

Within the framework of a functional integral formalism incorporating ionic charge and hard-core (HC) interactions on an equal footing, we formulate a unified theory of equilibrium thermodynamics and ion association in charged solutions.…

Soft Condensed Matter · Physics 2026-02-02 Sahin Buyukdagli

Motivated by SYK-like models describing near-BPS black holes in string/M-theory, we consider gauging the U$(1)$ symmetry of the complex SYK model in the presence of a Wilson line with charge $k$. At a fixed background gauge field, solutions…

High Energy Physics - Theory · Physics 2025-10-10 Ziruo Zhang , Cheng Peng

We analyze the mathematically rigorous BIBEE (boundary-integral based electrostatics estimation) approximation of the mixed-dielectric continuum model of molecular electrostatics, using the analytically solvable case of a spherical solute…

Computational Engineering, Finance, and Science · Computer Science 2015-05-30 Jaydeep P. Bardhan , Matthew G. Knepley

A density functional theory for a macroion suspension is examined, where the excess free energy corresponds to the macroion self energy arising from the polarisation of the supporting electrolyte solution. This is treated within a…

Soft Condensed Matter · Physics 2007-05-23 Patrick B. Warren

Recently, underscreening in concentrated electrolytes was discovered in experiments and confirmed in simulations and theory. It was found that the correlation length of the charge-charge correlations, $\lambda_s$, satisfies the scaling…

Statistical Mechanics · Physics 2022-11-07 A. Ciach , O. Patsahan

Thermodynamic properties of charge-stabilised colloidal suspensions are commonly modeled by implementing the mean-field Poisson-Boltzmann (PB) theory within a cell model. This approach models a bulk system by a single macroion, together…

Soft Condensed Matter · Physics 2015-05-18 Alan R. Denton

A model of dense plasmas relying on the superconfiguration approximation is presented. In each superconfiguration the nucleus is totally screened by the electrons in a Wigner-Seitz sphere (ion-sphere model). Superconfigurations of the same…

Atomic Physics · Physics 2007-06-26 Jean-Christophe Pain

An effective theory to treat the dense nuclear medium by the perturbative expansion method is proposed as a natural extension of the Heavy Baryon Chiral Perturbation Theory (HBChPT). Treating the Fermi momentum scale as a separate scale of…

High Energy Physics - Phenomenology · Physics 2007-05-23 Masayasu Harada , Dong-Pil Min , Tae-Sun Park , Chihiro Sasaki , Chaejun Song

We formulate an extension of the Debye-Hueckel-Bjerrum theory [M. E. Fisher and Y. Levin, Phys. Rev. Lett. 71, 3826 (1993)] to the fluid state of a highly asymmetric charged colloid. Allowing for the formation of clusters consisting of one…

Soft Condensed Matter · Physics 2015-06-25 M. N. Tamashiro , Yan Levin , Marcia C. Barbosa

The aim of this paper is to analyze from a mathematical perspective some existing schemes to partition a molecular density into several atomic contributions, with a specific focus on Iterative Stockholder Atom (ISA) methods. We provide a…

Numerical Analysis · Mathematics 2022-05-11 Robert Benda , Eric Cancès , Virginie Ehrlacher , Benjamin Stamm

We illustrate the main features of a recently proposed method based on ensemble density functional theory to divide rigorously a complex molecular system into its parts [M.H. Cohen and A. Wasserman, J. Phys. Chem. A 111, 2229 (2007)]. The…

Other Condensed Matter · Physics 2016-09-28 Morrel H. Cohen , Adam Wasserman , Kieron Burke

The Debye-H\" uckel formula for ionic activity coefficients is extended for concentrated solutions by solving a simple model of many-body Coulomb correlations and adding the Born solvation energy. Given the bulk permittivity, our formula is…

Chemical Physics · Physics 2017-09-12 Sven Schlumpberger , Martin Z. Bazant

Electrostatic correlation effects in inhomogeneous symmetric electrolytes are investigated within a previously developed electrostatic self-consistent (SC) theory (R.R. Netz and H. Orland, Eur. Phys.J. E 11, 301 (2003)). To this aim, we…

Soft Condensed Matter · Physics 2015-06-05 Sahin Buyukdagli , Cristian Achim , Tapio Ala-Nissila

We derive a Debye-H\"uckel-like model of the electric ion-ion interaction for non-constant dielectric susceptibility, which does not depend on any kind of charging process due to its foundation in the general framework of non-equilibrium…

Chemical Physics · Physics 2025-02-24 Wolfgang Dreyer , Rüdiger Müller

Density functional theory for a simple model of dendrimers is proposed. The theory is based on fundamental measure theory which accounts for the hard-sphere repulsion of the segments and on the Wertheim first-order perturbation theory for…

Soft Condensed Matter · Physics 2012-11-12 Alexandr Malijevsky

A theoretical analysis of Coulomb systems on lattices in general dimensions is presented. The thermodynamics is developed using Debye-Huckel theory with ion-pairing and dipole-ion solvation, specific calculations being performed for 3D…

Statistical Mechanics · Physics 2009-11-07 Vladimir Kobelev , Anatoly B. Kolomeisky , Michael E. Fisher