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We report the discovery of a spin one diamond lattice in NiRh2O4. This spinel undergoes a cubic to tetragonal phase transition at T = 440 K that leaves all nearest neighbor interactions equivalent. In the tetragonal phase, magnetization…

Strongly Correlated Electrons · Physics 2018-03-30 J. R. Chamorro , L. Ge , J. Flynn , M. Subramanian , M. Mourigal , T. M. McQueen

Frustration in spin system can give rise to unique ordered states and as a consequence several physical phenomena are expected such as multiferroics, high temperature superconductors and anomalous hall effect. Here we report the "new…

Strongly Correlated Electrons · Physics 2018-08-01 GiBaik Sim , SungBin Lee

Magnetization plateaux, visible as anomalies in magnetic susceptibility at low temperatures, are one of the hallmarks of frustrated magnetism. An extremely robust half-magnetization plateau is observed in the spinel oxides CdCr2O4 and…

Strongly Correlated Electrons · Physics 2007-06-06 Nic Shannon , Hiroaki Ueda , Yukitoshi Motome , Karlo Penc , Hiroyuki Shiba , Hidenori Takagi

Frustrated magnetic systems exhibit highly degenerate ground states and strong fluctuations, often leading to new physics. An intriguing example of current interest is the antiferromagnet on a diamond lattice, realized physically in A-site…

Materials Science · Physics 2011-09-21 G. J. MacDougall , D. Gout , J. L. Zarestky , G. Ehlers , A. Podlesnyak , M. A. McGuire , D. Mandrus , S. E. Nagler

Frustrated systems are ubiquitous and interesting because their behavior is difficult to predict. Magnetism offers extreme examples in the form of spin lattices where all interactions between spins cannot be simultaneously satisfied. Such…

Strongly Correlated Electrons · Physics 2009-11-07 S. -H. Lee , C. Broholm , W. Ratcliff , G. Gasparovic , Q. Huang , T. H. Kim , S. -W. Cheong

The collective behavior of interacting magnetic moments can be strongly influenced by the topology of the underlying lattice. In geometrically frustrated spin systems, interesting chiral correlations may develop that are related to the spin…

Strongly Correlated Electrons · Physics 2007-05-23 D. Grohol , K. Matan , J. H. Cho , S. -H. Lee , J. W. Lynn , D. G. Nocera , Y. S. Lee

On a lattice composed of triangular plaquettes where antiferromagnetic exchange interactions between localized spins cannot be simultaneously satisfied, the system becomes geometrically frustrated with magnetically disordered phases…

Geometrical frustration is a central challenge in contemporary condensed matter physics, a crucible favourable to the emergence of novel physics. The pyrochlore magnets, with rare earth magnetic moments localized at the vertices of…

Strongly Correlated Electrons · Physics 2015-05-30 Sylvain Petit , Pierre Bonville , Isabelle Mirebeau , Hannu Mutka , Julien Robert

In antiferromagnets, the interplay of spin frustration and spin-lattice coupling has been extensively studied as the source of complex spin patterns and exotic magnetism. Here, we demonstrate that, although neglected in the past, the…

Dynamical properties of the lattice structure was studied by optical spectroscopy in ACr2O4 chromium spinel oxide magnetic semiconductors over a broad temperature region of T=10-335K. The systematic change of the A-site ions (A=Mn, Fe, Co,…

Strongly Correlated Electrons · Physics 2013-07-24 V. Kocsis , S. Bordács , D. Varjas , K. Penc , A. Abouelsayed , C. A. Kuntscher , K. Ohgushi , Y. Tokura , I. Kézsmárki

The standard approach to realize a spin liquid state is through magnetically frustrated states, relying on ingredients such as the lattice geometry, dimensionality, and magnetic interaction type of the spins. While Heisenberg spins on a…

Strongly Correlated Electrons · Physics 2025-04-10 Margarita G. Dronova , Vaclav Petricek , Zachary Morgan , Feng Ye , Daniel M. Silevitch , Yejun Feng

We consider some classical and frustrated lattice spin models with global O(3) spin symmetry. There is no general analytical method to find a ground-state if the spin dependence of the Hamiltonian is more than quadratic (i.e. beyond the…

Strongly Correlated Electrons · Physics 2015-03-17 Laura Messio , Claire Lhuillier , Grégoire Misguich

The $A$-site spinel NiRh$_2$O$_4$ is the only known realization of a spin-1 diamond lattice magnet and is predicted to host unconventional magnetic phenomena driven by frustrated nearest and next-nearest neighbor exchange as well as orbital…

Strongly Correlated Electrons · Physics 2022-08-10 B. Zager , J. R. Chamorro , L. Ge , V. Bisogni , J. Pelliciari , J. Li , G. Fabbris , T. M. McQueen , M. Mourigal , K. W. Plumb

ZnCr2O4 undergoes a first order spin-Peierls-like phase transition at 12.5 K from a cubic spin liquid phase to a tetragonal Neel state. Using powder diffraction and single crystal polarized neutron scattering, we determined the complex spin…

Strongly Correlated Electrons · Physics 2009-11-13 S. -H. Lee , W. Ratcliff , Q. Huang , T. H. Kim , S-W. Cheong

In the spinel compound GeCo$_2$O$_4$, the Co$^{2+}$ pyrochlore sublattice presents remarkable magnetic field-induced behaviors that we unveil through neutron and X-ray single-crystal diffraction. The N\'eel ordered magnetic phase is entered…

Strongly Correlated Electrons · Physics 2017-02-01 X. Fabrèges , E. Ressouche , F. Duc , S. de Brion , M. Amara , C. Detlefs , L. Paolasini , E. Suard , L. -P. Regnault , B. Canals , P. Strobel , V. Simonet

The inversion and volume effects on magnetism in a spinel-type magnetically frustrated compound, CoAl2O4, and its gallium-substituted system, CoAl2-xGaxO4, were investigated. Magnetically frustrated Co2+ with spin S = 3/2 on the tetrahedral…

We present a systematic inelastic neutron scattering and neutron diffraction study of the magnetic structure of the quasi-1D spin-1/2 magnet SrCo2V2O8, where the interchain coupling in the Neel-type antiferromagnetic ground state breaks the…

Strongly Correlated Electrons · Physics 2022-03-04 L. Shen , E. Campillo , O. Zaharko , P. Steffens , M. Boehm , K. Beauvois , B. Ouladdiaf , Z. He , D. Prabhakaran , A. T. Boothroyd , E. Blackburn

Using synchrotron X-rays and neutron diffraction we disentangle spin-lattice order in highly frustrated ZnCr$_2$O$_4$ where magnetic chromium ions occupy the vertices of regular tetrahedra. Upon cooling below 12.5 K the quandary of…

Strongly Correlated Electrons · Physics 2009-05-14 S. Ji , S. -H. Lee , C. Broholm , T. Y. Koo , W. Ratcliff , S-W. Cheong , P. Zschack

The ferrimagnetic spinel MnCr2S4 shows a variety of magnetic-field-induced phase transitions owing to bond frustration and strong spin-lattice coupling. However, the site-resolved magnetic properties at the respective field-induced phases…

Strongly Correlated Electrons · Physics 2021-02-17 Sh. Yamamoto , H. Suwa , T. Kihara , T. Nomura , Y. Kotani , T. Nakamura , Y. Skourski , S. Zherlitsyn , L. Prodan , V. Tsurkan , H. Nojiri , A. Loidl , J. Wosnitza

The crystal and magnetic structures of stoichiometric ZnCr2Se4 have been investigated using synchrotron X-ray and neutron powder diffraction, muon spin relaxation (muSR) and inelastic neutron scattering. Synchrotron X-ray diffraction shows…

Strongly Correlated Electrons · Physics 2017-04-12 P. Zajdel , W-Y. Li , W. Van Beek , A. Lappas , A. Ziolkowska , S. Jaskiewicz , C. Stock , M. A. Green
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