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Neutron and X-ray diffraction, magnetic susceptibility, and specific heat measurements have been used to investigate the magnetic and structural phase transitions of the spinel system Fe1+xCr2-xO4(0.0<=x<=1.0). The temperature versus Fe…

The mutual coupling of spin and lattice degrees of freedom is ubiquitous in magnetic materials and potentially creates exotic magnetic states in response to the external magnetic field. Particularly, geometrically frustrated magnets serve…

Ag2CrO2 is an S=3/2 frustrated triangular lattice antiferromagnet without orbital degree of freedom. With decreasing temperature, a 4-sublatice spin state develops. However, a long-range partially disordered state with 5 sublattices…

Strongly Correlated Electrons · Physics 2012-04-13 M. Matsuda , H. Yoshida , M. Isobe , C. de la Cruz , R. S. Fishman

We review the mechanism of spin-lattice coupling in relieving the geometrical frustration of pyrochlore antiferromagnets, in particular spinel oxides. The tetrahedral unit, which is the building block of the pyrochlore lattice, undergoes a…

Strongly Correlated Electrons · Physics 2018-07-25 O. Tchernyshyov , G. -W. Chern

The competition between interactions in frustrated magnets allows a wide variety of new ground states, often exhibiting emergent physics and unique excitations. Expanding the suite of lattices available for study enhances our chances of…

Strongly Correlated Electrons · Physics 2017-01-24 Darren C. Peets , Hasung Sim , Seongil Choi , Maxim Avdeev , Seongsu Lee , Su Jae Kim , Hoju Kang , Docheon Ahn , Je-Geun Park

We determined the magnetic structure of CuCr$_2$O$_4$ using neutron diffraction and irreducible representation analysis. The measurements identified a new phase between 155 K and 125 K as nearly collinear magnetic ordering in the Cr…

Strongly Correlated Electrons · Physics 2018-03-20 K. Tomiyasu , S. Lee , H. Ishibashi , Y. Takahashi , T. Kawamata , Y. Koike , T. Nojima , S. Torii , T. Kamiyama

We demonstrate via a muon spin rotation experiment that the electronic ground state of the iridium spinel compound, CuIr$_2$S$_4$, is not the presumed spin-singlet state but a novel paramagnetic state, showing a quasistatic spin glass-like…

Strongly Correlated Electrons · Physics 2014-02-27 K. M. Kojima , 2 R. Kadono , M. Miyazaki , M. Hiraishi , I. Yamauchi , A. Koda , Y. Tsuchiya , H. S. Suzuki , H. Kitazawa

In the highly frustrated pyrochlore magnet spins form a lattice of corner sharing tetrahedra. We show that the tetrahedral ``molecule'' at the heart of this structure undergoes a Jahn-Teller distortion when lattice motion is coupled to the…

Strongly Correlated Electrons · Physics 2007-05-23 Oleg Tchernyshyov , R. Moessner , S. L. Sondhi

Magnetic frustration is a route that can lead to the emergence of novel ground states, including spin liquids and spin ices. Such frustration can be introduced through either the geometry of lattice structures or by incompatible exchange…

The spin-lattice coupling plays an important role in strongly frustrated magnets. In ZnCr$_2$O$_4$, an excellent realization of the Heisenberg antiferromagnet on the ``pyrochlore'' network, a lattice distortion relieves the geometrical…

Strongly Correlated Electrons · Physics 2009-11-10 A. B. Sushkov , H. D. Drew , O. Tchernyshyov , W. Ratcliff , S. W. Cheong

While the dominant magnetic interaction in La$_2$CuO$_4$ is superexchange between nearest-neighbor Cu moments, the pinning of the spin direction depends on weak anisotropic effects associated with spin-orbit coupling. The symmetry of the…

Strongly Correlated Electrons · Physics 2023-03-17 Xiao Hu , A. Sapkota , V. O. Galea , G. D. Gu , I. A. Zaliznyak , J. M. Tranquada

Insulating spinel materials, with the chemical formula $AB_2X_4$, behave as diamond lattice antiferromagnets when only the A-site atom is magnetic. Many exhibit classic signatures of frustration, induced not geometrically but by competing…

Strongly Correlated Electrons · Physics 2011-11-15 SungBin Lee , Leon Balents

We present an elaborate electron-spin resonance study of the low-energy dynamics and magnetization in the ordered phase of the magnetically frustrated spinel ZnCr$_2$O$_4$. We observe several resonance modes corresponding to different…

Strongly Correlated Electrons · Physics 2010-11-29 V. N. Glazkov , A. M. Farutin , V. Tsurkan , H. -A. Krug von Nidda , A. Loidl

We studied temperature and magnetic field dependence of magnetization, $M(T)$ and $M(B)$, on thiospinel FeCr$_{2}$S$_{4}$. We observed a step-like anomaly at $T_{OO} \sim$ 9 K for $M$($T$) attributed to an orbital order transition in…

Strongly Correlated Electrons · Physics 2015-05-28 Masakazu Ito , Yuji Nagi , Naotoshi Kado , Shinpei Urakawa , Takuro Ogawa , Akihiro Kondo , Keiichi Koyama , Kazuo Watanabe , Koichi Kindo

We re-investigate the magnetically frustrated, {\it diamond-lattice-antiferromagnet} spinels FeAl$_2$O$_4$ and MnAl$_2$O$_4$ using magnetization measurements and diffuse scattering of polarized neutrons. In FeAl$_2$O$_4$, macroscopic…

Disordered Systems and Neural Networks · Physics 2015-06-19 Harikrishnan S. Nair , Zhendong Fu , Jörg Voigt , Yixi Su , Th. Brückel

Magnetic ordering in the geometrically frustrated magnetic oxide spinels MgCr_2O_4 and ZnCr_2O_4 is accompanied by a structural change that helps relieve the frustration. Analysis of high-resolution synchrotron X-ray scattering reveals that…

Frustration refers to competition between different interactions that cannot be simultaneously satisfied, a familiar feature in many magnetic solids. Strong frustration results in highly degenerate ground states, and a large suppression of…

Strongly Correlated Electrons · Physics 2007-07-03 Doron Bergman , Jason Alicea , Emanuel Gull , Simon Trebst , Leon Balents

Ca3Ru2O7 is a correlated and spin-orbit-coupled system with an extraordinary anisotropy. It is both interesting and unique largely because this material exhibits conflicting phenomena that are often utterly inconsistent with traditional…

Strongly Correlated Electrons · Physics 2021-10-04 Hengdi Zhao , Hao Zheng , Jasminka Terzic , Wenhai Song , Yifei Ni , Yu Zhang , Pedro Schlottmann , Gang Cao

Compounds of the new materials class LnTAl$_4$X$_2$ (Ln = lanthanide, X = tetrel, T = transition metal) host exotic magnetic phenomena due to geometric frustration induced by their triangular lattice. Complex spin arrangements, magnetic…

A novel general method of describing the spin-lattice interactions in magnetic solids was proposed in terms of first principles calculations. The spin exchange and Dzyaloshinskii-Moriya interactions as well as their derivatives with respect…

Strongly Correlated Electrons · Physics 2011-12-30 H. J. Xiang , E. J. Kan , Su-Huai Wei , M. -H. Whangbo , X. G. Gong