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We study the spin chain behavior, a transition to 3D magnetic order and the magnitudes of the exchange interactions for the metal-amino acid complex Cu(D,L-alanine)2.H2O, a model compound to investigate exchange couplings supported by…

Mesoscale and Nanoscale Physics · Physics 2016-03-22 Rafael Calvo , Rosana P. Sartoris , Hernan L. Calvo , Edson F. Chagas , Raul E. Rapp

The magnetic phase diagram and the thermodynamic properties of a square lattice containing antiferromagnetically coupled spin-1/2 triangles are studied. A Heisenberg Hamiltonian with three strong intra-triangle exchange coupling constants…

Strongly Correlated Electrons · Physics 2009-10-31 Stefan Wessel , Stephan Haas

The properties of two molecular-based magnetic helices, composed of 3$d$ metal Co and Mn ions bridged by Nitronyl Nitroxide radicals, are investigated by density functional calculations. Their peculiar and distinctive magnetic behavior is…

Materials Science · Physics 2015-05-20 Marco Scarrozza , Alessandro Vindigni , Paolo Barone , Roberta Sessoli , Silvia Picozzi

We have studied in details the electronic structure and magnetism in M (Mn and Cr) doped semiconducting half-Heusler compounds FeVSb, CoTiSb and NiTiSn (XM$_{x}$Y$_{1-x}$Z) in a wide concentration range using local-spin density functional…

Materials Science · Physics 2007-05-23 B. R. K. Nanda , I. Dasgupta

We have investigated the structural and magnetic transitions in CsCoO$_2$ using calorimetric measurements, neutron powder diffraction (NPD), density functional theory (DFT) calculations and muon-spin relaxation ($\mu$SR) measurements.…

Strongly Correlated Electrons · Physics 2015-06-23 N. Z. Ali , R. C. Williams , F. Xiao , S. J. Clark , T. Lancaster , S. J. Blundell , D. V. Sheptyakov , M. Jansen

The spin-1/2 alternating Heisenberg chain system Na$_3$Cu$_2$SbO$_6$ features two relevant exchange couplings: $J_{1a}$ within the structural Cu$_2$O$_6$ dimers and $J_{1b}$ between the dimers. Motivated by the controversially discussed…

Strongly Correlated Electrons · Physics 2014-11-13 M. Schmitt , O. Janson , S. Golbs , M. Schmidt , W. Schnelle , J. Richter , H. Rosner

Within a first principles framework, we study the electronic structure of the recently synthesized polymeric coordination compound Cu(II)-2,5-bis(pyrazol-1-yl)-1,4-dihydroxybenzene (CuCCP), which has been suggested to be a good realization…

We report on high-field magnetization, specific-heat and electron spin resonance (ESR) studies of the quasi-two-dimensional spin-1/2 Heisenberg antiferromagnet [Cu(pyz)2(HF2)]PF6. The frequency-field diagram of ESR modes below TN = 4.38 K…

Strongly Correlated Electrons · Physics 2011-03-10 E. Cizmar , S. A. Zvyagin , R. Beyer , M. Uhlarz , M. Ozerov , Y. Skourski , J. L. Manson , J. A. Schlueter , J. Wosnitza

The new antiferromagnetic (AF) compound BaCu_2Si_2O_7 is studied by magnetic susceptibility and neutron scattering techniques. The observed behavior is dominated by the presence of loosely coupled S=1/2 chains with the intrachain AF…

Strongly Correlated Electrons · Physics 2007-05-23 I. Tsukada , Y. Sasago , K. Uchinokura , A. Zheludev , S. Maslov , G. Shirane , K. Kakurai , E. Ressouche

We report synthesis and magnetic properties of quasi-one-dimensional spin-$\frac{1}{2}$ Heisenberg antiferromagnetic chain compound BaNa$_2$Cu(VO$_4$)$_2$. This orthovanadate has a centrosymmetric crystal structure, $C2/c$, where the…

We present a combined experimental and theoretical study of the spin-1/2 compound CuP$_2$O$_6$ that features a network of two-dimensional (2D) antiferromagnetic (AFM) square planes, interconnected via one-dimensional (1D) AFM spin chains.…

We present a comprehensive investigation of the intricate spin dynamics in the non-centrosymmetric compound Sm$_7$Pd$_3$, revealing the coexistence of spin glass, domain glass, and ferromagnetic (FM) behaviors. Magnetic field-dependent…

Materials Science · Physics 2025-05-15 Ajay Kumar , Anis Biswas , Yaroslav Mudryk

The magnetic properties of the ferromagnetic-ferromagnetic-antiferromagnetic trimerized spin-1/2 Heisenberg chain are studied theoretically. The high temperature susceptibilty and the ground state saturation magnetic field are calculated…

Condensed Matter · Physics 2009-10-22 Kazuo Hida

Neutron spectroscopy measurements have been performed on single crystals of the antiferromagnetic van der Waals compound NiPS$_3$. Linear spin wave theory using a Heisenberg Hamiltonian with single-ion anisotropies has been applied to…

Strongly Correlated Electrons · Physics 2022-12-19 A. R. Wildes , J. R. Stewart , M. D. Le , R. A. Ewings , K. C. Rule , G. Deng , K. Anand

In conventional quasi-one-dimensional antiferromagnets with quantum spins, magnetic excitations are carried by either magnons or spinons in different energy regimes: they do not coexist independently, nor could they interact with each…

Strongly Correlated Electrons · Physics 2020-07-30 H. Zhang , Z. Zhao , D. Gautreau , M. Raczkowski , A. Saha , V. O. Garlea , H. Cao , T. Hong , H. O. Jeschke , Subhendra D. Mahanti , T. Birol , F. F. Assaad , X. Ke

We have successfully synthesized S = 1/2 kagome antiferromagnets MCu3(OH)6Cl2 (M = Ni and Co) by hydrothermal method with rotating pressure vessel. Structural characterization shows that both compounds have the similar crystal structure as…

Strongly Correlated Electrons · Physics 2012-12-10 Yue-sheng Li , Qing-ming Zhang

1H nuclear magnetic resonance (NMR) measurements in [YPc2]0, an organic compound formed by radicals stacking along chains, are presented. The temperature dependence of the macroscopic susceptibility, of the NMR shift and of the spin-lattice…

Strongly Correlated Electrons · Physics 2015-05-20 F. Branzoli , P. Carretta , M. Filibian , S. Klyatskaya , M. Ruben

We show that the magnetism of double perovskite AFe_{1/2}M_{1/2}O_3 systems may be described by the Heisenberg model on the simple cubic lattice, where only half of sites are occupied by localized magnetic moments. The nearest-neighbor…

Materials Science · Physics 2015-01-16 R. O. Kuzian , I. V. Kondakova , A. -M. Dare , V. V. Laguta

The spin-1/2 Ising-Heisenberg branched chain, inspired by the magnetic structure of three isostructural polymeric coordination compounds [(Tp)2Fe2(CN)6X(bdmap)Cu2(H2O)].H2O to be further denoted as Fe2Cu2 (Tp = tris(pyrazolyl)hydroborate,…

Statistical Mechanics · Physics 2024-09-10 David Sivy , Katarina Karlova , Jozef Strecka

We present self flux growth and characterization of single crystalline AlMn$_2$B$_2$. It is an orthorhombic (space group Cmmm), layered material with a plate like morphology. The anisotropic bulk magnetization data, electrical transport and…

Materials Science · Physics 2019-07-03 Tej N. Lamichhane , Khusboo Rana , Qisheng Lin , Sergey L. Bud'ko , Yuji Furukawa , Paul C. Canfield