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We investigate the structural and magnetic properties of the new quantum magnet BaCuTe$_2$O$_6$. This compound is synthesized for the first time in powder and single crystal form. Synchrotron X-ray and neutron diffraction reveal a cubic…

Strongly Correlated Electrons · Physics 2021-03-17 A. Samartzis , D. Khalyavin , A. T. M. N. Islam , S. Chillal , K. Siemensmeyer , K. Prokes , D. J. Voneshen , A. Senyshyn , B. Lake

The chain-like system Ba_{3}Cu_{3}Sc_4O_{12} has potentially interesting magnetic properties due to the presence of Cu^{2+} and a structure-suggested low-dimensionality. We present magnetization M versus magnetic field H and temperature T,…

Strongly Correlated Electrons · Physics 2012-11-16 B. Koteswararao , A. V. Mahajan , F. Bert , P. Mendels , J. Chakraborty , V. Singh , I. Dasgupta , S. Rayaprol , V. Siruguri , A. Hoser , S. D. Kaushik

We calculate the magnetic interactions between two nearest neighbor substitutional magnetic ions (Co or Mn) in ZnO by means of density functional theory and compare it with the available experimental data. Using the local spin density…

Materials Science · Physics 2007-05-23 Thomas Chanier , M. Sargolzaei , I. Opahle , R. Hayn , K. Koepernik

We present comprehensive high magnetic field studies of the alternating weakly coupled ferro-antiferromagnetic (FM-AFM) spin-$1/2$ chain compound Cu$_2$(OH)$_3$Br, with the structure of the natural mineral botallackite. Our measurements…

Strongly Correlated Electrons · Physics 2024-12-17 K. Yu. Povarov , Y. Skourskii , J. Wosnitza , D. E. Graf , Z. Zhao , S. A. Zvyagin

Using the first-principles density functional approach, we investigate a material Pr$_2$MgIrO$_6$ (PMIO) of double perovskite structure synthesized recently. According to the calculations, PMIO is a magnetic Mott-Hubbard insulator…

Materials Science · Physics 2016-04-29 Madhav P. Ghimire , Long-Hua Wu , Xiao Hu

Using thermodynamic measurements and density-functional band-structure calculations, we explore magnetic behavior of SrCuTe2O6. Despite being a structural sibling of a three-dimensional frustrated system PbCuTe2O6, this spin-1/2 quantum…

Materials Science · Physics 2015-06-29 N. Ahmed , A. A. Tsirlin , R. Nath

From experimental and theoretical analyses of magnetic and specific-heat properties, we present the complete magnetic phase diagram of the quasi-one-dimensional antiferromagnet Cu(N$_2$H$_5$)$_2$(SO$_4$)$_2$. On cooling and at zero magnetic…

Strongly Correlated Electrons · Physics 2016-11-23 A. Paduan-Filho , A. P. Vieira , J. G. A. Ramon , R. S. Freitas

This work reports the synthesis, structure and magnetic properties of the single crystal of a facile spin 1/2 one dimensional Heisenberg antiferromagnet bis(4-aminopyridinium) bis(oxalato)cuprate(II) dihydrate, (C 5 H 7 N 2 ) 2 [Cu(C 2 O 4…

The magnetic structure of the edge sharing cuprate compound Li2CuO2 has been investigated by means of ab initio electronic structure calculations. The first and second neighbor in-chain magnetic interactions are calculated to be -142 K and…

Materials Science · Physics 2007-05-23 Coen de Graaf , Iberio de P. R. Moreira , Francesc Illas , Oscar Iglesias , Amilcar Labarta

We investigate the structural and magnetic properties of two molecule-based magnets synthesized from the same starting components. Their different structural motifs promote contrasting exchange pathways and consequently lead to markedly…

Hybrid density functional calculations are performed for a variety of systems containing d9 ions (Cu2+, Ag2+), and exhibiting quasi-one-dimensional magnetic properties. In particular we study fluorides containing these ions in a rarely…

Strongly Correlated Electrons · Physics 2017-11-01 Dominik Kurzydlowski , Wojciech Grochala

We studied structural and magnetic properties of a series of insulating double perovskite compounds, La$_{2-x}$Sr$_{x}$CuRuO$_{6}$ (0 $\le$ x $\le$ 1), representing doping via \textit{A}-site substitution. The end members…

Strongly Correlated Electrons · Physics 2012-09-19 P. Anil Kumar , R. Mathieu , R. Vijayaraghavan , Subham Majumdar , Olof Karis , P. Nordblad , Biplab Sanyal , Olle Eriksson , D. D. Sarma

We present a theoretical and experimental study of a quasi-one-dimensional zigzag antiferromagnet (N_2H_5)CuCl_3, which can be viewed as weakly coupled Heisenberg chains with a frustrated interaction. We first discuss generic features of…

Strongly Correlated Electrons · Physics 2009-11-07 N. Maeshima , M. Hagiwara , Y. Narumi , K. Kindo , T. C. Kobayashi , K. Okunishi

A microscopic magnetic model for the spin-1/2 Heisenberg chain compound CuSe2O5 is developed based on the results of a joint experimental and theoretical study. Magnetic susceptibility and specific heat data give evidence for quasi-1D…

Strongly Correlated Electrons · Physics 2009-11-20 O. Janson , W. Schnelle , M. Schmidt , Yu. Prots , S. -L. Drechsler , S. K. Filatov , H. Rosner

The atomic and magnetic structures of (Cu$X$)LaNb$_2$O$_7$ ($X$=Cl and Br) are investigated using the density-functional calculations. Among several dozens of examined structures, an orthorhombic distorted $2\times 2$ structure, in which…

Strongly Correlated Electrons · Physics 2015-05-14 Chung-Yuan Ren , Ching Cheng

The structure and the magnetic properties of layered Li3Cu2SbO6 are investigated by powder X-ray diffraction, static susceptibility, and electron spin resonance studies up to 330 GHz. The XRD data experimentally verify the space group C2/m…

Magnetism in Ni-Mn-Z (Z = Ga,In,Sn,Sb) Heusler alloys has so far been predominantly attributed to Rudermann-Kittel-Kasuya-Yoshida type interactions between Mn atoms. We investigate magnetic interactions in one such alloy,…

Materials Science · Physics 2015-06-15 K. R. Priolkar , P. A. Bhobe , D. N. Lobo , S. W. D'Souza , S. R. Barman , A. Chakrabarti , S. Emura

We investigate the microscopic origin of the ferromagnetic and antiferromagnetic spin exchange couplings in the quasi one-dimensional cobalt compound Ca3Co2O6. In particular, we establish a local model which stabilizes a ferromagnetic…

Strongly Correlated Electrons · Physics 2009-11-10 Raymond Frésard , Christian Laschinger , Thilo Kopp , Volker Eyert

The title compounds have dominant ferromagnetic (FM) exchange interactions within one-dimensional (1D) half-twist ladders of s =1/2 Cu2^{+} ions and antiferromagnetic(AFM) interactions between ladders, leading to ordered 3D phases at…

Strongly Correlated Electrons · Physics 2015-06-15 M. Kumar , S. E. Dutton , R. J. Cava , Z. G. Soos

The first-principles full-potential linearized augmented plane-wave method based on density functional theory is used to investigate electronic structure and magnetic properties of hypothetical binary compounds of I$^{A}$ subgroup elements…

Materials Science · Physics 2008-09-14 Krzysztof Zberecki , Leszek Adamowicz , Michał Wierzbicki