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We demonstrate a compact technique to compress electron pulses to attosecond length, while keeping the energy spread reasonably small. The technique is based on Dielectric Laser Acceleration (DLA) in nanophotonic silicon structures. Unlike…

Accelerator Physics · Physics 2021-02-17 Uwe Niedermayer , Dylan S. Black , Kenneth J. Leedle , Yu Miao , Robert L. Byer , Olav Solgaard

The motion of electrons in or near solids, liquids and gases can be tracked by forcing their ejection with attosecond x-ray pulses, derived from femtosecond lasers. The momentum of these emitted electrons carries the imprint of the…

Mesoscale and Nanoscale Physics · Physics 2017-06-14 C. W. Barlow-Myers , N. J. Pine , W. A. Bryan

We theoretically study how time- and angle-resolved photoemission spectroscopy can be applied for imaging coherent electron dynamics in molecules. We consider a process in which a pump pulse triggers coherent electronic dynamics in a…

Optics · Physics 2018-12-11 Daria Popova-Gorelova , Jochen Küpper , Robin Santra

A compact high repetition rate attosecond light source based on a standard laser oscillator combined with plasmonic enhancement is presented. At repetition rates of tens of MHz, we predict focusable pulses with durations of ~< 300…

Optics · Physics 2014-05-19 Mattia Lupetti , Matthias F. Kling , Armin Scrinzi

We investigate ionization of neon atoms by an isolated attosecond pump pulse in the presence of two coherent extreme ultraviolet or x-ray probe fields. The probe fields are tuned to a core-valence transition in the residual ion and induce…

Atomic Physics · Physics 2016-03-30 Jhih-An You , Nina Rohringer , Jan Marcus Dahlström

Attosecond chemistry involves developing strategies to manipulate electronic coherent waves in molecules, which can influence the outcome of photoinduced reactions. While recent progress in this field calls for investigations of…

Chemical Physics · Physics 2026-04-22 Evan Munaro-Langloÿs , Franck Lépine , Victor Despré

Coherent control over electron dynamics in atoms and molecules using high-intensity circularly-polarized laser pulses gives rise to current loops, resulting in the emission of magnetic fields. We propose and demonstrate with ab-initio…

We introduce and experimentally demonstrate a method, where the two intrinsic time scales of a molecule, the slow nuclear motion and the fast electronic motion, are simultaneously measured in a photo-electron photo-ion coincidence…

In this tutorial we provide a short review of attosecond pulse characterization techniques and a pedagogical account of a recently proposed method called Pulse Analysis by Delayed Absorption (PANDA) [Pabst and Dahlstr\"om, Phys. Rev. A, 94,…

Quantum Physics · Physics 2018-11-26 Jan Marcus Dahlström , Stefan Pabst , Eva Lindroth

In this manuscript we present a theoretical framework and its numerical implementation to simulate the out-of-equilibrium electron dynamics induced by the interaction of ultrashort laser pulses in condensed-matter systems. Our approach is…

Recent advances in attosecond spectroscopy techniques have fueled the interest in the theoretical description of electronic processes taking place in the subfemtosecond time scale. Here we study the coupled dynamic screening of a localized…

Atomic and Molecular Clusters · Physics 2013-01-28 N. E. Koval , D. Sánchez-Portal , A. G. Borisov , R. Díez Muiño

We numerically investigate the use of strong THz radiation in assisting single attosecond pulse generation by few-cycle, 800 nm laser pulses. We optimize focusing conditions to generate short and powerful single attosecond pulses of…

Optics · Physics 2014-02-14 Emeric Balogh , Katalin Kovács , Valer Tosa , Katalin Varjú

An electrical pulse E(t) is completely defined by its time-dependent amplitude and polarisation direction. For optical pulses the manipulation and characterisation of the light polarisation state is fundamental due to its relevance in…

Light-matter interactions are of fundamental scientific and technological interest. Ultrafast electron microscopy and diffraction with combined femtosecond-nanometer resolution elucidate the laser-induced dynamics in structurally…

Materials Science · Physics 2025-04-08 Till Domröse , Leonardo da Camara Silva , Claus Ropers

Photoelectron interferometry with femto- and atto-second light pulses is a powerful probe of the fast electron wavepacket dynamics, albeit it has practical limitations on the energy resolution. We show that one can simultaneously obtain…

Atomic Physics · Physics 2022-02-24 A. Plunkett , M. A. Alarcon , J. K. Wood , C. H. Greene , A. Sandhu

The ionization dynamics of a Xenon cluster with 40 atoms is analyzed under a pum p probe scenario of laser pulses where an infrared laser pulse of 50 fs length follows with a well defined time delay a VUV pulse of the same length and peak…

Atomic and Molecular Clusters · Physics 2009-11-10 Ch. Siedschlag , J. M. Rost

Attosecond transient-absorption spectroscopy (ATAS) is an established method for exploring electron dynamics on the subfemtosecond time-scale. ATAS spectra contain certain ubiquitous features, such as oscillating fringes, light-induced…

Atomic Physics · Physics 2017-08-02 Jørgen Johansen Rørstad , Jens E. Bækhøj , Lars Bojer Madsen

We propose a protocol to probe the ultrafast evolution and dephasing of coherent electronic excitation in molecules in the time domain by the intrinsic streaking field generated by the molecule itself. Coherent electronic motion in the…

Development of ultrafast lasers and non-linear optical techniques over the last two decades provides tools to access real-time dynamics of low energy excitations in superconductors. For example, time-resolved THz spectroscopy and time- and…

Superconductivity · Physics 2022-04-20 Jure Demsar