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Coherent light pulses of few to hundreds of femtoseconds (fs) duration have prolifically served the field of ultrafast phenomena. While fs pulses address mainly dynamics of nuclear motion in molecules or lattices in the gas, liquid or…

Chemical Physics · Physics 2013-04-26 P. A. Carpeggiani , P. Tzallas , A. Palacios , D. Gray , F. Martín , D. Charalambidis

We study laser-assisted photodetachment time delays by attosecond pulse trains from the closed-shell negative ions F- and Cl-. We investigate the separability of the delay into two contributions: (i) the Wigner-like delay associated with…

Atomic Physics · Physics 2017-09-13 Eva Lindroth , Jan Marcus Dahlström

Ultrashort electron bunches are useful for applications like ultrafast imaging and coherent radiation production. Currently, however, the shortest achievable bunches, at attosecond time scales, have only been realized in the single or very…

Accelerator Physics · Physics 2019-04-19 J. Lim , Y. D. Chong , L. J. Wong

The feasibility of generation of bright ultrashort gamma-ray pulses is demonstrated in the interaction of a relativistic electron bunch with a counterpropagating tightly-focused superstrong laser beam in the radiation dominated regime. The…

Atomic Physics · Physics 2015-11-11 Jian-Xing Li , Karen Z. Hatsagortsyan , Benjamin J. Galow , Christoph H. Keitel

Determining the pulse duration of femtosecond electron bunches is challenging and often experimentally invasive. An effective method for measuring the duration based on the time-dependent variations in electron beam divergence induced by a…

Accelerator Physics · Physics 2025-07-01 Andreas Seidel , Carola Zepter , Alexander Sävert , Stephan Kuschel , Matt Zepf

With the generation of high order harmonics (HHG) on the plasma surface it is possible to turn the laser pulse into a train of attosecond or even zeptosecond pulses in the back radiation. These attosecond pulses may have amplitude several…

Plasma Physics · Physics 2015-12-17 Mykyta Cherednychek , Alexander Pukhov

We report on the first streaking measurement of water-window attosecond pulses generated via high harmonic generation, driven by sub-2-cycle, CEP-stable, 1850 nm laser pulses. Both the central photon energy and the energy bandwidth far…

Time-resolved studies have so far relied on rapidly triggering a photo-induced dynamic in chemical or biological ions or molecules and subsequently probing them with a beam of fast moving photons or electrons that crosses the studied…

Chemical Physics · Physics 2021-03-19 Hazem Daoud , R. J. Dwayne Miller

Extreme-ultraviolet pulses can propagate through ionised solid-density targets, unlike optical pulses and, thus, have the potential to probe the interior of such plasmas on sub-femtosecond timescales. We present a synthetic diagnostic…

Plasma Physics · Physics 2022-04-27 Andréas Sundström , István Pusztai , Per Eng-Johnsson , Tünde Fülöp

Electronic correlations occur on attosecond timescales, dictating how chemical bonds form, energy flows, and materials respond to light. Capturing such many-body processes requires light pulses of similar duration. The soft X-ray water…

Linear off-resonant X-ray Raman techniques are capable of detecting the ultrafast electronic coherences generated when a photoexcited wave packet passes through a conical intersection. A hybrid femtosecond or attosecond probe pulse is…

Chemical Physics · Physics 2022-11-07 Lorenzo Restaino , Deependra Jadoun , Markus Kowalewski

We demonstrate experimentally the isolation of single attosecond pulses at the carbon K- shell edge in the soft-X-ray water window. Attosecond pulses at photon energies that cover the principal absorption edges of the building blocks of…

Attosecond streaking is one of the most fundamental processes in attosecond science allowing for a mapping of temporal (i.e. phase) information on the energy domain. We show that on the single-particle level attosecond streaking time shifts…

We find a solution of the wave equation in the paraxial approximation that describes the attosecond pulses with spatiotemporal helical structure in the phase and in the intensity recently generated by means of highly nonlinear optical…

Optics · Physics 2019-09-25 Miguel A. Porras

We report on the observation, characterization, and control of the electron dynamics in ionized argon atoms. We utilized an intense mid-infrared (MIR) pulse to create a coherent superposition of the spin-orbit split ground state of the ion.…

Electrical pulse stimulation drives many important physical phenomena in condensed matter as well as in electronic systems and devices. Often, nanoscopic and mesoscopic mechanisms are hypothesized, but methods to image electrically driven…

Mesoscale and Nanoscale Physics · Physics 2023-06-05 Thomas E Gage , Daniel B Durham , Haihua Liu , Supratik Guha , Ilke Arslan , Charudatta Phatak

Half-cycle picosecond pulses have been produced from thin photo-conductors, when applying an electric field across the surface and switching on conduction by a short laser pulse. Then the transverse current in the wafer plane emits…

Optics · Physics 2015-06-03 H. -C. Wu , J. Meyer-ter-Vehn

Dielectric laser acceleration is a versatile scheme to accelerate and control electrons with the help of femtosecond laser pulses in nanophotonic structures. We demonstrate here the generation of a train of electron pulses with individual…

Accelerator Physics · Physics 2020-01-29 Norbert Schönenberger , Anna Mittelbach , Peyman Yousefi , Uwe Niedermayer , Peter Hommelhoff

Ultrafast laser excitation can create coherent superpositions of electronic states in molecules and trigger ultrafast flow of electron density on few- to sub-femtosecond time scales. While recent attosecond experiments have addressed…

Chemical Physics · Physics 2020-11-18 Yuki Kobayashi , Daniel M. Neumark , Stephen R. Leone

A new regime in the interaction of a two-colour ($\omega$,$2\omega$) laser with a nanometre-scale foil is identified, resulting in the emission of extremely intense, isolated attosecond pulses - even in the case of multi-cycle lasers. For…

Plasma Physics · Physics 2020-04-22 Y. X. Zhang , S. Rykovanov , Mingyuan Shi , C. L. Zhong , X. T. He , B. Qiao , M. Zepf