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Single-molecule electronics has been envisioned as the ultimate goal in the miniaturisation of electronic circuits. While the aim of incorporating single-molecule junctions into modern technology still proves elusive, recent developments in…

Mesoscale and Nanoscale Physics · Physics 2017-11-22 Jakub K. Sowa , Jan A. Mol , G. Andrew D. Briggs , Erik M. Gauger

We study the conductance of an interconnect between two graphene leads formed by a single-atom carbon chain. Its dependence on the chemical potential and the number of atoms in the chain is qualitatively different from that in the case of…

Mesoscale and Nanoscale Physics · Physics 2011-09-12 Wei Chen , A. V. Andreev , G. F. Bertsch

Using a break junction technique, we find a clear signature for the formation of conducting hybrid junctions composed of a single organic molecule (benzene, naphthalene or anthracene) connected to chains of platinum atoms. The hybrid…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 Tamar Yelin , Ran Vardimon , Natalia Kuritz , Richard Korytár , Alexei Bagrets , Ferdinand Evers , Leeor Kronik , Oren Tal

We present a theory of single-electron tunneling transport through a ferromagnetic nanoparticle in which particle-hole excitations are coupled to spin collective modes. The model employed to describe the interaction between quasiparticles…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 L. Michalak , C. M. Canali , V. G. Benza

The electron transport in a four-terminal nanodevice consisting of two crossed nanotubes is investigated in the framework of the Landauer-Buttiker formalism. The evident formula for the ballistic conductance of the device is found using a…

Mesoscale and Nanoscale Physics · Physics 2011-11-09 Viktor Margulis , Mikhail Pyataev

We report on scanning tunneling microscopy (STM) topographs of individual metal phthalocyanines (MPc) on a thin salt (NaCl) film on a gold substrate, at tunneling energies within the molecule's electronic transport gap. Theoretical models…

Mesoscale and Nanoscale Physics · Physics 2023-10-24 Abhishek Grewal , Christopher C. Leon , Klaus Kuhnke , Klaus Kern , Olle Gunnarsson

The effect on molecular transport due to chemical modification of the metal-molecule interface is investigated, using as an example the prototypical molecular device formed by attaching a p-disubstituted benzene molecule onto two gold…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Yongqiang Xue , Mark A. Ratner

We analyze the electronic transport through a model spin-1 molecule as a function of temperature, magnetic field and bias voltage. We consider the effect of magnetic anisotropy, which can be generated experimentally by stretching the…

Strongly Correlated Electrons · Physics 2011-06-24 P. S. Cornaglia , P. Roura Bas , A. A. Aligia , C. A. Balseiro

Vibrationally coupled electron transport through single-molecule junctions is considered. Reviewing our recent theoretical work, we show that electron-hole pair creation processes represent the key to understand the vibrational excitation…

Mesoscale and Nanoscale Physics · Physics 2013-11-13 R. Härtle , U. Peskin , M. Thoss

Electronic transport across n-Si-alkyl monolayer/Hg junctions is, at reverse and low forward bias, independent of alkyl chain-length from 18 down to 1 or 2 carbons! This and further recent results indicate that electron transport is…

We examine electron transport through a single-molecule magnet Mn12 bridged between Au electrodes using the first-principles method. We find crucial features which were inaccessible in model Hamiltonian studies: spin filtering and a strong…

Materials Science · Physics 2015-05-14 Salvador Barraza-Lopez , Kyungwha Park , Victor Garcia-Suarez , Jaime Ferrer

We report on the effect of sp3 hybridized carbon atoms in acene derivatives adsorbed on metal surfaces, namely decoupling the molecules from the supporting substrates. In particular, we have used a Ag(100) substrate and hydrogenated…

We present a simple and reliable method for making electrical contacts to small organic molecules with thiol endgroups. Nanometer-scale gaps between metallic electrodes have been fabricated by passing a large current through a…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Subhasis Ghosh , Henny Halimun , Jaewon Choi , Saurabh Lodha , David Janes

Nanoelectronics requires the development of a priori technology evaluation for materials and device design that takes into account quantum physical effects and the explicit chemical nature at the atomic scale. Here, we present a…

Mesoscale and Nanoscale Physics · Physics 2013-06-04 Dimpy Sharma , Lida Ansari , Baruch Feldman , Marios Iakovidis , James Greer , Giorgos Fagas

Understanding of charge transport mechanisms in nanoscale structures is essential for the development of molecular electronic devices. Charge transport through 1D molecular systems connected between two contacts is influenced by several…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Daijiro Nozaki , Horacio M. Pastawski , Gianaurelio Cuniberti

If simple guidelines could be established for understanding how quantum interference (QI) can be exploited to control the flow of electricity through single molecules, then new functional molecules, which exploit room-temperature QI could…

Mesoscale and Nanoscale Physics · Physics 2019-03-11 Lara Ulčakar , Tomaž Rejec , Jure Kokalj , Sara Sangtarash , Hatef Sadeghi , Anton Ramšak , John H. Jefferson , Colin J. Lambert

For investigation of electron transport on the nanoscale, a system possessing a simple to interpret electronic structure is composed of alkane chains bridging two electrodes via end groups; to date the majority of experiments and…

Materials Science · Physics 2007-10-01 Giorgos Fagas , James C. Greer

Electron transport through a single-level quantum dot weakly coupled to Luttinger liquid leads is considered in the master equation approach. It is shown that for a weak or moderately strong interaction the differential conductance…

Strongly Correlated Electrons · Physics 2013-02-06 G. A. Skorobagatko , I. V. Krive

Building upon traditional quantum chemistry calculations, we have implemented an {\em ab-initio} method to study the electrical transport in nanocontacts. We illustrate our technique calculating the conductance of C$_{60}$ molecules…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. J. Palacios , A. J. Perez-Jimenez , E. Louis , J. A. Verges

We identify the leading processes of electron transport across finite-length segments of proximitized nanowires and build a quantitative theory of their two-terminal conductance. In the presence of spin-orbit interaction, a nanowire can be…

Mesoscale and Nanoscale Physics · Physics 2016-06-28 B. van Heck , R. M. Lutchyn , L. I. Glazman