Related papers: Generating Unexpected Spin Echoes in Dipolar Solid…
In spectroscopy, it is conventional to treat pulses much stronger than the linewidth as delta-functions. In NMR, this assumption leads to the prediction that pi pulses do not refocus the dipolar coupling. However, NMR spin echo measurements…
The present work is a comment on PRL 98, 190401 (2007), arXiv:0705.0667 . The authors reported NMR measurements in solids with different pulse sequences. In some multiple $\pi$ pulse echo trains they observed coherent signals of several…
NMR spin echo measurements of $^{29}$Si in Silicon powders have uncovered a variety of surprising phenomena that appear to be independent of doping. These surprises include long tails and even-odd asymmetry in Carr-Purcell-Meiboom-Gill…
Puzzling anomalies previously observed in multipulse NMR experiments in natural abundance 29Si [A.E. Dementyev, D. Li, K. MacLean, and S.E. Barrett, Phys. Rev. B 68, 153302 (2003)] such as long-lived spin echoes and even-odd asymmetries,…
We report an observation of extremely long-lived spin states in systems of dipolar-coupled nuclear spins in solids. The 'suspended echo' experiment uses a simple stimulated echo pulse sequence and creates non-equilibrium states which live…
The application of Carr-Purcell-Meiboom-Gill (CPMG) $\pi-$trains for dynamically decoupling a system from its environment has been extensively studied in a variety of physical systems. When applied to dipolar solids, recent experiments have…
We demonstrate that CPMG and XYXY decoupling sequences with non-ideal $\pi$ pulses can reduce dipolar interactions between spins of the same species in solids. Our simulations of pulsed electron spin resonance (ESR) experiments show that…
The reversal of the time evolution of the local polarization in an interacting spin system involves a sign change of the effective dipolar Hamiltonian which refocuses the 'spin diffusion' process generating a polarization echo. Here, the…
Dense spin ensembles in solids present a natural platform for studying quantum many-body dynamics. Multiple-pulse coherent control can be used to manipulate the magnetic dipolar interaction between the spins to engineer their dynamics.…
I describe composite pulses during which the average dipolar interactions within a spin ensemble are controlled while realizing a global rotation. The construction method used is based on the average Hamiltonian theory and rely on the…
The tiny difference between hard pi pulses and their delta-function approximation can be exploited to control coherence. Variants on the magic echo that work despite a large spread in resonance offsets are demonstrated using the zeroth- and…
Silicon is promising for spin-based quantum computation because nuclear spins, a source of magnetic noise, may be eliminated through isotopic enrichment. Long spin decoherence times, $T_2$, have been measured in isotope-enriched silicon but…
We note the existence of a set of magnetic field values where a simple Hahn echo sequence refocuses the dynamics of the full dipolar interaction, for spin systems of electron donors in silicon. As the refocussing occurs for both arbitrary…
Pulsars are famed for their rotational clock-like stability and their highly-repeatable pulse shapes. However, it has long been known that there are unexplained deviations (often termed "timing noise") from the rate at which we predict…
Pulsed electrically-detected magnetic resonance of phosphorous (31P) in bulk crystalline silicon at very high magnetic fields (B > 8.5 T) and low temperatures (T = 2.8 K) is presented. We find that the spin-dependent capture and reemission…
The anomalous magnetic and electric dipole moments in spin motion equation acquire pseudoscalar corrections if the $T(CP)$-noninvariance is admitted. It allows to explain the discrepancy between experimental and theoretical values of muon…
Quantum unitary evolution typically leads to thermalization of generic interacting many-body systems. There are very few known general methods for reversing this process, and we focus on the magic echo, a radio-frequency pulse sequence…
Theoretical treatment of the electron spin echo envelope modulation (ESEEM) spectra from polarons in a semiconducting $\pi$- conjugated polymer is presented. The contact hyperfine coupling and the dipolar interaction between the polaron and…
Most materials freeze when cooled to sufficiently low temperature. We find that magnetic dipoles randomly distributed in a solid matrix condense into a spin liquid with spectral properties on cooling that are the diametric opposite of those…
The evolution of local spin polarization in finite systems involves interference phenomena that give rise to {\bf quantum dynamical echoes }and non-ergodic behavior. We predict the conditions to observe these echoes by exploiting the NMR…