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We review the magnetic and orbital ordered states in \cro{} by performing Resonant Elastic X-ray Scattering (REXS) at the Ru L$_{2,3}$-edges. In principle, the point symmetry at Ru sites does not constrain the direction of the magnetic…

Strongly Correlated Electrons · Physics 2018-09-27 D. G. Porter , V. Granata , F. Forte , S. Di Matteo , M. Cuoco , R. Fittipaldi , A. Vecchione , A. Bombardi

We investigate the orbital fluctuations in the ferromagnetic-metallic phase of La$_{1.2}$Sr$_{1.8}$Mn$_2$O$_7$ by considering a two orbital model within a tight-binding description which reproduces the ARPES Fermi surface. We find strong…

Strongly Correlated Electrons · Physics 2017-06-29 Dheeraj Kumar Singh , Ki Hoon Lee , Tetsuya Takimoto

The emergence of superlattice periodicities at metal to insulator transitions in hole doped perovskite oxides responds to a rearrangement of the local atomic structure, and electron and spin density distribution. Originally, the ionic model…

Strongly Correlated Electrons · Physics 2015-05-14 Javier Herrero-Martin , Joaquín García , Blasco Javier , Claudio Mazzoli , G. Subías

The ground-state orbital occupancy of the Ru$^{4+}$ ion in Ca$_{2-x}$La$_x$RuO$_4$ [x=0, 0.05(1), 0.07(1) and 0.12(1)] was investigated by performing X-ray absorption spectroscopy (XAS) in the vicinity of the O K edge as a function of angle…

Strongly Correlated Electrons · Physics 2019-02-13 D. Pincini , L. S. I. Veiga , C. D. Dashwood , F. Forte , M. Cuoco , R. S. Perry , P. Bencok , A. T. Boothroyd , D. F. McMorrow

Magnetization measurements of URu2Si2 in pulsed magnetic fields of 44 T reveal that the hidden order phase is destroyed before appearing in the form of a re-entrant phase between ~ 36 and 39 T. Evidence for conventional itinerant electron…

Strongly Correlated Electrons · Physics 2009-11-10 N. Harrison , M. Jaime , J. A. Mydosh

We explore orbital dynamics in the spin liquid candidate Ba3CuSb2O9 using multi-frequency electron spin resonance. We prepared two high quality single crystals. The crystal with a slight copper deficiency shows a structural phase transition…

Strongly Correlated Electrons · Physics 2015-12-09 Yibo Han , Masayuki Hagiwara , Takehito Nakano , Yasuo Nozue , Kenta Kimura , Mario Halim , Satoru Nakatsuji

The local and intermediate structure of stoichiometric LaMnO$_3$ has been studied in the pseudocubic and rhombohedral phases at high temperatures (300 to 1150 K). Neutron powder diffraction data were collected and a combined Rietveld and…

Strongly Correlated Electrons · Physics 2009-11-10 Xiangyun Qiu , Th. Proffen , J. F. Mitchell , S. J. L. Billinge

We have experimentally found related anomalies in electrical resistivity, dc and ac magnetic susceptibility, appearing deeply within ferromagnetically ordered state in SrRuO3. Lack of Jahn-Teller distortion in this regime rules out…

Strongly Correlated Electrons · Physics 2008-06-27 I. M. Bradaric , M. S. Laad , F. V. Kusmartsev , K. Yoshii , S. Okayasu

La doped SrFeO$_{3}$, La$_{1/3}$Sr$_{2/3}$FeO$_{3}$, exhibits a metal-to-insulator transition accompanied by both antiferromagnetic and charge ordering states along with the Fe-O bond disproportionation below a critical temperature near…

Strongly Correlated Electrons · Physics 2025-06-25 Nam Nguyen , Alex Taekyung Lee , Vijay Singh , Anh T. Ngo , Hyowon Park

To understand the orbital ordering of $LaMnO_3$ in the ground state, we study it in the A-type spin antiferromagnetic state. We calculate the two-dimensional response functions associated with the Jahn-Teller $Q_2$ and $Q_3$ distortions and…

Strongly Correlated Electrons · Physics 2007-05-23 Sudhakar Yarlagadda , Manidipa Mitra

We studied the charge-orbital ordering in the superlattice of charge-ordered insulating Pr$_{0.5}$Ca$_{0.5}$MnO$_3$ and ferromagnetic metallic La$_{0.5}$Sr$_{0.5}$MnO$_3$ by resonant soft x-ray diffraction. A temperature-dependent…

Strongly Correlated Electrons · Physics 2014-08-07 H. Wadati , J. Okamoto , M. Garganourakis , V. Scagnoli , U. Staub , M. Nakamura , M. Kawasaki , Y. Tokura

Measurements of the electrical and thermal conductivities, thermopower and paramagnetic susceptibility have been performed on single crystal samples of Bi1/2Sr1/2MnO3 and complemented with the X-ray powder diffraction data. A pronounced…

Strongly Correlated Electrons · Physics 2009-11-07 J. Hejtmanek , K. Knizek , Z. Jirak , M. Hervieu , C. Martin , M. Nevriva , P. Beran

We study long wavelength magnetic excitations in lightly doped La_{2-x}Sr_{x}CuO_{4} (x < 0.03) detwinned crystals. The lowest energy magnetic anisotropy induced gap can be understood in terms of the antisymmetric spin interaction inside…

Strongly Correlated Electrons · Physics 2009-11-10 A. Gozar , B. S. Dennis , G. Blumberg , Seiki Komiya , Yoichi Ando

For the paramagnetic insulating phase in the metal-ordered manganite YBaMn2O6, the so-called CE-type of charge/orbital ordered state was observed within the monoclinic ab-plane, which is most commonly observed for the ordinary half doped…

Strongly Correlated Electrons · Physics 2009-11-07 H. Kageyama , T. Nakajima , M. Ichihara , Y. Ueda , H. Yoshizawa , K. Ohoyama

We report resonant x-ray scattering studies of charge and orbital order in Pr_{1-x}Ca_{x}MnO_3 with x=0.4 and 0.5. Below the ordering temperature, T_O=245 K, the charge and orbital order intensities follow the same temperature dependence,…

Strongly Correlated Electrons · Physics 2009-10-31 M. v. Zimmermann , J. P. Hill , Doon Gibbs , M. Blume , D. Casa , B. Keimer , Y. Murakami , Y. Tomioka , Y. Tokura

We investigated the electronic structure of the enigmatic CeRh$_3$B$_2$ using resonant inelastic scattering and x-ray absorption spectroscopy in combination with $ab$ $initio$ density functional calculations. We find that the Rh 4$d$ states…

The ferroelectric (Sm C$^*$) -- antiferroelectric (Sm C$^*_A$) -- reentrant ferroelectric (re Sm C$^*$) phase temperature sequence was observed for system with competing synclinic - anticlinic interactions. The basic properties of this…

Soft Condensed Matter · Physics 2009-10-31 D. Pociecha , E. Gorecka , M. Cepic , N. Vaupotic , B. Zeks , D. Kardas , J. Mieczkowski

For the past decades, the low-temperature phase of Ca$_3$Ru$_2$O$_7$ below the 48K first-order phase transition remains a puzzle with controversial suggestions involving metallic ferroelectric, orbital or magnetic ordering. Through analysis…

Strongly Correlated Electrons · Physics 2018-09-13 Zheting Jin , Wei Ku

We review our recent x-ray scattering studies of charge and orbital order in doped manganites, with specific emphasis on the role of orbital correlations in Pr_1-xCa_xMnO_3. For x=0.25, we find an orbital structure indistinguishable from…

We present powder and single crystal X-ray diffraction data as evidence for a monoclinic distortion in the low spin (S=0) and intermediate spin state (S=1) of LaCoO3. The alternation of short and long bonds in the ab plane indicates the…

Strongly Correlated Electrons · Physics 2009-11-10 G. Maris , Y. Ren , V. Volotchaev , C. Zobel , T. Lorenz , T. T. M. Palstra