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We demonstrate that the onset of complex spin orders in ACr$_2$O$_4$ spinels with magnetic A$=$Co, Fe and Cu ions lowers the lattice symmetry. This is clearly indicated by the emergence of anisotropic lattice dynamics -- as evidenced by the…

Strongly Correlated Electrons · Physics 2014-01-15 S. Bordacs , D. Varjas , I. Kezsmarki , G. Mihaly , L. Baldassarre , A. Abouelsayed , C. A. Kuntscher , K. Ohgushi , Y. Tokura

We studied in detail the low temperature/high magnetic field phases of URu$_{2}$Si$_{2}$ single crystals with specific heat, magnetocaloric effect, and magnetoresistance in magnetic fields up to 45 T. Data obtained down to 0.5 K, and…

Strongly Correlated Electrons · Physics 2009-11-07 M. Jaime , K. H. Kim , G. Jorge , S. McCall , J. A Mydosh

Resonant x-ray emission spectroscopy (RXES) was employed at the U L3 absorption edge and the La1 emission line to explore the 5f occupancy, nf, and the degree of 5f orbital delocalization in the hidden order compound URu2Si2. By comparing…

Strongly Correlated Electrons · Physics 2016-08-03 C. H. Booth , S. A. Medling , J. G. Tobin , R. E. Baumbach , E. D. Bauer , D. Sokaras , D. Nordlund , T. -C. Weng

The alkaline-earth orthovanadate Sr$_3$V$_2$O$_8$ with the palmierite structure is reported to host a dielectric anomaly as well as a structural phase transition above the room temperature. With V$^{5+}$ ions and tetrahedral oxygen…

Materials Science · Physics 2023-11-28 Amartyajyoti Saha , Turan Birol

The crystalline and magnetic structures of Ca$_2$Ru$_{1-x}$Fe$_x$O$_4$ (x=0.02, 0.05, 0.08 and 0.12) have been studied using neutron and X-ray diffraction. The Fe-doping reduces the Ru-O bond length in both apical and planar directions. The…

Strongly Correlated Electrons · Physics 2020-07-31 Songxue Chi , Feng Ye , Gang Cao , Huibo Cao , Jaime A. Fernandez-Baca

Common wisdom dictates that physical systems become less ordered when heated to higher temperature. However, several systems display the opposite phenomenon and move to a more ordered state upon heating, e.g. at low temperature…

Disordered Systems and Neural Networks · Physics 2024-08-13 Flaviano Morone , Dries Sels

Recently the Ce-based caged-type compounds having general formula CeT2Al10 (T=Fe, Ru and Os) have generated considerable interest due to the Kondo semiconducting paramagnetic ground state (down to 40 mK) observed in CeFe2Al10 and…

Strongly Correlated Electrons · Physics 2015-06-18 D. T. Adroja , A. D. Hillier , Y. Muro , T. Takabatake , A. M. Strydom , A. Bhattacharyya , A. Daoud-Aladin , J. W. Taylor

The Ce$^{3+}$ pseudospin-1/2 degrees of freedom in Ce$_2$Zr$_2$O$_7$ possess both dipolar and octupolar character which enables the possibility of novel quantum spin liquid ground states in this material. Here we report new muon spin…

Neutron inelastic scattering and diffraction techniques have been used to study the MnV2O4 spinel system. Our measurements show the existence of two transitions to long-range ordered ferrimagnetic states; the first collinear and the second…

Strongly Correlated Electrons · Physics 2009-11-13 V. O. Garlea , R. Jin , D. Mandrus , B. Roessli , Q. Huang , M. Miller , A. J. Schultz , S. E. Nagler

In Ca1-xRExFeAs2 (RE= rare earth), an antiferromagnetic (AFM) phase as well as a structural transition has been reported, even in the electron-overdoped regime. Here we investigated the temperature-dependent in-plane optical spectroscopy of…

Superconductivity · Physics 2016-06-15 Run Yang , Bing Xu , Yaomin Dai , Wei Zhang , Jinyun Liu , Ziyang Qiu , Xianggang Qiu

We report evidence for a reentrant spin glass phase in electron-doped $\text{EuFe}_2\text{As}_2$ single crystals and first traces of the superconductivity re-entrance in optics. In the close-to-optimal doped…

Superconductivity · Physics 2017-06-07 A. Baumgartner , D. Neubauer , S. Zapf , A. V. Pronin , W. H. Jiao , G. H. Cao , M. Dressel

Microstructure properties, phase transitions, and charge ordering in the LuFe2O4 materials have been extensively investigated by means of transmission electron microscopy (TEM). The (001) twins as a common defect frequently appear in the…

Strongly Correlated Electrons · Physics 2007-05-23 Y. Zhang , H. X. Yang , C. Ma , H. F. Tian , J. Q. Li *

The candidate magnetoelectric Pb3Mn7O15 has a structure consisting of 1/3 filled Kagome layers linked by ribbons of edge-sharing octahedra in the stacking direction. Previous reports have indicated a complex hexagonal-orthorhombic…

Strongly Correlated Electrons · Physics 2012-04-18 Simon A. J. Kimber

When holes are doped into a Mott-Hubbard type insulator, like lightly doped manganites of the La(1-x)CaxMnO3 family, the cooperative Jahn-Teller distortions and the appearance of orbital ordering require an arrangement of Mn(3+)/Mn(4+) for…

Strongly Correlated Electrons · Physics 2009-11-10 G. Papavassiliou , M. Pissas , M. Belesi , M. Fardis , J. P. Ansermet , D. Carlier , C. Dimitropoulos , J. Dolinsek

We investigated the temperature ($T=$ 15 $\sim $ 290 K) and the magnetic field ($H=$ 0 $\sim $ 17 T) dependent optical conductivity spectra of a charge/orbital ordered manganite, Nd$_{1/2}$Sr$_{1/2}$MnO$_3$. With variation of $T$ and $H$,…

Strongly Correlated Electrons · Physics 2009-10-31 J. H. Jung , H. J. Lee , T. W. Noh , E. J. Choi , Y. Moritomo , Y. J. Wang , X. Wei

A second-order phase transition is associated with emergence of an "order parameter" and a spontaneous symmetry breaking. For the heavy fermion superconductor URu$_2$Si$_2$, the symmetry of the order parameter associated with its ordered…

Strongly Correlated Electrons · Physics 2015-04-30 H. -H. Kung , R. E. Baumbach , E. D. Bauer , V. K. Thorsmølle , W. -L. Zhang , K. Haule , J. A. Mydosh , G. Blumberg

We investigate the electronic, magnetic and orbital properties of La0.5Ca0.5MnO3 perovskite by means of an ab initio electronic structure calculation within the Hartree-Fock approximation. Using the experimental crystal structure reported…

Strongly Correlated Electrons · Physics 2009-11-10 V. Ferrari , M. D. Towler , P. B. Littlewood

We consider the orbital ordering in LaMnO3 and similar systems, proceeding from the band picture. We show that for the realistic magnetic structure of A-type there exists a complete nesting betweeen two e_g-bands. As a result there occurs…

Strongly Correlated Electrons · Physics 2009-11-10 D. V. Efremov , D. I. Khomskii

When matter is cooled from high temperatures, collective instabilities develop amongst its constituent particles that lead to new kinds of order. An anomaly in the specific heat is a classic signature of this phenomenon. Usually the…

Strongly Correlated Electrons · Physics 2009-11-07 P. Chandra , P. Coleman , J. A. Mydosh , V. Tripathi

Sr3(Ru1-xMnx)2O7, in which 4d-Ru is substituted by the more localized 3d-Mn, is studied by x-ray dichroism and spin-resolved density functional theory. We find that Mn impurities do not exhibit the same 4+ valence of Ru, but act as 3+…

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