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Forty-five years after the point de d\'epart [1] of density functional theory, its applications in chemistry and the study of electronic structures keep steadily growing. However, the precise form of the energy functional in terms of the…

Chemical Physics · Physics 2019-10-29 Philippe Blanchard , José M. Gracia-Bondía , Joseph C. Várilly

The ionization of a one-dimensional model Helium atom in short laser pulses using time-dependent density functional theory is investigated. We calculate ionization probabilities as a function of laser intensity by approximating the…

Atomic Physics · Physics 2009-11-13 F. Wilken , D. Bauer

Inspired by earlier work on the band-gap problem in insulators, we reexamine the treatment of strongly correlated Hubbard-type models within density-functional theory. In contrast to previous studies, the density is fully parametrized by…

Strongly Correlated Electrons · Physics 2008-02-03 Arno Schindlmayr , R. W. Godby

We study the impact of the multi-lepton searches at the LHC on supersymmetric models with compressed mass spectra. For such models the acceptances of the usual search strategies are significantly reduced due to requirement of large…

High Energy Physics - Phenomenology · Physics 2015-06-05 Krzysztof Rolbiecki , Kazuki Sakurai

The density functional scheme for calculating the pair density is presented by means of the constrained-search technique. The resultant single-particle equation takes the form of the modified Hartree-Fock equation which contains the kinetic…

Strongly Correlated Electrons · Physics 2015-06-25 Masahiko Higuchi , Katsuhiko Higuchi

The electron localization function (ELF) is a universal measure of electron localization that allows for, e.g., an effective characterization of physical bonds in molecular and solid state systems. In the context of the widely used…

Strongly Correlated Electrons · Physics 2019-08-20 Alexander Lindmaa , Joel Davidsson , Ann E. Mattsson , Rickard Armiento

In the present communication the Bayesian conditional probability approach is applied to the wave function of a many-electron system that results in appearance of a quantum vector potential in the DFT Schrodinger equation due to electron…

Chemical Physics · Physics 2012-12-05 R. Tsekov , G. N. Vayssilov

It is believed that, in the limit as the conductor tends to infinity, correlations between the zeros of elliptic curve $L$-functions averaged within families follow the distribution laws of the eigenvalues of random matrices drawn from the…

Number Theory · Mathematics 2008-11-17 D. K. Huynh , J. P. Keating , N. C. Snaith

We observe that a system of irreducible, fiber-linear, first class constraints on T*M is equivalent to the definition of a foliation Lie algebroid over M. The BFV formulation of the constrained system is given by the Hamiltonian lift of the…

Mathematical Physics · Physics 2019-02-20 Noriaki Ikeda , Thomas Strobl

We prove that the electron density function of a real physical system can be uniquely determined by its values on any finite subsystem. This establishes the existence of a rigorous density-functional theory for any open electronic system.…

Quantum Physics · Physics 2007-05-23 Xiao Zheng , Fan Wang , GuanHua Chen

A generalization of the Kohn--Sham approach is derived where the correlation-energy functional depends on the one-particle density matrix of noninteracting states and on the external potential from the interacting target-state. The…

Chemical Physics · Physics 2007-05-23 James P. Finley

In the recent work of S. Sharma \emph{et al.}, (arxiv.org: arxiv:0912.1118), a single-electron spectrum associated with the natural orbitals was defined as the derivative of the total energy with respect to the occupation numbers at half…

Chemical Physics · Physics 2012-03-07 E. N. Zarkadoula , S. Sharma , J. K. Dewhurst , E. K. U. Gross , N. N. Lathiotakis

The Debye-H\" uckel formula for ionic activity coefficients is extended for concentrated solutions by solving a simple model of many-body Coulomb correlations and adding the Born solvation energy. Given the bulk permittivity, our formula is…

Chemical Physics · Physics 2017-09-12 Sven Schlumpberger , Martin Z. Bazant

A curious behavior of electron correlation energy is explored. Namely, the correlation energy is the energy that tends to drive the system toward that of the uniform electron gas. As such, the energy assumes its maximum value when a…

Materials Science · Physics 2019-12-17 Teepanis Chachiyo , Hathaithip Chachiyo

It is shown that the electron density functional correlation functional satisfies an equation that links the N-electron and (N-1)-electron densities of the same adiabatically scaled Hamiltonian of the interacting electron system.

Materials Science · Physics 2012-04-01 Daniel P. Joubert

Accurately describing strong electron correlation in complex systems remains a prominent challenge in computational chemistry as near-term quantum algorithms treating total correlation often require prohibitively deep circuits. Here we…

Computational Engineering, Finance, and Science · Computer Science 2026-04-21 Zhanou Liu , Yuhao Chen , Yingjin Ma , Xiao He , Yuxin Deng

Exact density-functional theory is reconstructed here from its convex variational structure as two parallel exact ensemble hierarchies: an interacting hierarchy rooted in Lieb's ensemble formulation and a noninteracting hierarchy rooted in…

Chemical Physics · Physics 2026-05-01 Nan Sheng

We review and illustrate with several examples the connection between the search for lower bounds for the optimal constant in the Lieb-Oxford inequality and the optimal transport limit (or strictly-correlated-electrons limit) of density…

Chemical Physics · Physics 2022-03-29 Michael Seidl , Tarik Benyahia , Derk P. Kooi , Paola Gori-Giorgi

In modeling low-dimensional electronic nanostructures, the evaluation of the electron-electron interaction is a challenging task. Here we present an accurate and practical density-functional approach to the two-dimensional many-electron…

Strongly Correlated Electrons · Physics 2010-10-29 S. Pittalis , E. Rasanen

We implement the Heisenberg principle into the Constrained Molecular Dynamics (CoMD) model with a similar approach to the Pauli principle using the one-body occupation probability $\bar{f}_i$. Results of the modified and the original model…

Nuclear Theory · Physics 2019-07-10 K. Wang , A. Bonasera , H. Zheng , G. Q. Zhang , Y. G. Ma , W. Q. Shen