Atomic Physics
We investigate using optically trapped linear polyatomic molecules as probes of nuclear spin-dependent parity violation. The presence of closely spaced, opposite-parity $\ell$-doublets is a general feature of such molecules, allowing…
We examine the influence of a static dc electric field on Electromagnetically Induced Transparency (EIT) resonances that involve highly excited Rydberg states. Our focus is on how these resonances are altered when the relative orientation…
Compared to other stable isotopes of $\rm{Yb}^+$, $^{173}\rm{Yb}^+$ has a richer hyperfine structure, which leads to more favorable clock transitions, spectroscopic techniques for probing new physics, and more sophisticated quantum…
We investigate the feasibility of using high-harmonic generation (HHG) as a complementary probe of tunneling delay in strong-field ionization. By combining time--frequency analysis of HHG spectra obtained from full time-dependent…
Cold atoms are promising platforms for metrology and quantum computation, yet their many-body dynamics remains largely unexplored. We here investigate Rabi oscillations from optically-thick cold clouds, driven by high-intensity coherent…
The ionization potential (IP) of radium monofluoride (RaF) was measured to be 4.969(2)[10] eV, revealing a relativistic enhancement in the series of alkaline earth monofluorides. The results are in agreement with a relativistic…
Optically pumped atomic magnetometers (OPAMs) offer high sensitivity at room temperature and are increasingly considered for portable magnetic sensing in geomagnetic-field environments. Here we report a handheld-scale, single-beam scalar…
We present precision spectroscopy and isotope shift measurement of the ${}^1S_0 \leftrightarrow {}^3P_2$ clock transition in neutral ytterbium ($\mathrm{Yb}$) atoms. By revealing a magic wavelength at $905.4(2)$ nm, we successfully achieve…
We study real-time photoionization flux at the $3s$ Amusia-Cooper minimum (ACM) in argon using \textit{ab initio} simulations with the relativistic time-dependent configuration-interaction singles (RTDCIS) method in length (LG) and velocity…
Three-body F\"orster resonances controlled by a dc electric field are of interest for the implementation of three-qubit quantum gates with single atoms in optical traps using their laser excitation into strongly interacting Rydberg states.…
Doppler-broadening thermometry (DBT) can be used as a calibration-free primary reference suitable for practical applications, e.g. reliably measuring temperatures over long periods of time in environments where sensor retrieval is…
By simulating the real-time multielectron wavefunction with the multi-configurational time-dependent Hartree-Fock (MCTDHF) approach, we conduct an \textit{ab initio} study of the single-photon ionization process of a body-fixed water…
We consider the formation of cold ground-state polar molecules in a low vibrational level by laser fields. Starting from a pair of cold colliding atoms of dissimilar species, we propose a strategy consisting of three steps. In the first…
We investigate the formation of non-ground-state Bose-Einstein condensates within the mean-field description represented by the Gross-Pitaevskii equation (GPE). The objective is to form excited states of a condensate known as nonlinear…
We present the design and fabrication of an endcap-type Paul trap. The trap is designed for studies with Ca$^{+}$ and Yb$^{+}$. The design, fabrication process, and characterization are presented in detail with a focus on trapping a single…
Rydberg atoms represent a platform underpinning many recent developments in quantum computation, simulation, sensing, and metrology. They further facilitate optical nonlinearity at the single-photon level when coupled to photons propagating…
We report on the creation of $^{86}$Sr$_2$ molecules in the halo state and neighboring weakly bound states. Efficient molecule production via one-photon photoassociation relies on sufficient wavefunction overlap between the target…
We propose a broadband, femtosecond two-photon excitation scheme for efficient population transfer to the ultra-narrow linewidth $1s2s\ ^1S_0$ metastable state in helium. Using $120$ nm vacuum ultraviolet (VUV) femtosecond laser pulses, we…
We introduce a framework for resolving electron-hole dynamics within wavefunction-based multiconfigurational time-dependent Hartree-Fock (MCTDHF) theory. Central to this framework is a time-domain generalization of the extended Koopmans'…
We demonstrate a method for controlling the outcome of an ultracold chemical few-body reaction by redirecting a tunable fraction of reaction flux from one selected product channel to another one. In the reaction, three ultracold atoms…