Atomic Physics
We study the parity-violating electron-electron interaction mediated by the axion-like in the hexatomic molecule of a symmetric top type. The rich rovibrational behavior require electronic computations for multiple molecular configurations…
We demonstrate a delay-programmable two-color femtosecond source based on a chirped-seed noncollinear optical parametric amplifier. Introducing controlled dispersion into the seed enables spectral selection through pump-seed delay, allowing…
We study the isotopic dependence of collisional widths and shifts of the Hg clock transition $^1$S$_0$-$^3$P$_0$ perturbed by the Rb atoms in the temperature range from 1 nK to 1 K. For this purpose, we model the Born-Oppenheimer effective…
We propose a laser isotope separation mechanism in which selectivity arises from nuclear spin rather than isotope shifts, enabling the use of broadband ultrafast lasers. A Ramsey pulse sequence is applied to paramagnetic molecular…
We report on efficient rovibrational state-selective loading of single H$_2^+$ molecular ions into a cryogenic linear Paul trap using (2+1) resonance-enhanced multi-photon ionization (REMPI). The H$_2^+$ ions are created by resonant…
Optical clocks have achieved remarkable estimated fractional frequency uncertainties reaching the $10^{-18}$ level and below, enabling applications in fundamental physics, general relativity, and geodesy. However, the challenge of verifying…
We use coupled-channel calculations to explore the nature of near-threshold bound states in a simplified model of Rb+KRb. This is a prototype for systems with very strong coupling at short range and chaotic behavior for the short-range…
We present a comprehensive theoretical investigation of hyperfine-resolved excitation and detection of the low-energy isomeric state of $^{229}$Th in trapped $^{229}\mathrm{Th}^{3+}$ ions. Using a quantum master equation approach, we…
We use a $^{87}\text{Rb}$ atomic vapor, suitable for an optically-pumped magnetometer (OPM) in Earth-field conditions, to study the noise properties of three strategies for generating pulsed optical pumping. We compare a frequency-modulated…
Penning traps, renowned for their unparalleled precision in determining fundamental properties such as mass and magnetic moments, are cornerstone instruments in modern physics. Their applications span from nuclear structure studies to…
We present absolute frequency measurements of 2S_{1/2}-nS_{1/2} two-photon transitions with n = 8, 9, and 10 in a cryogenic beam of atomic hydrogen. Each transition has been measured with a fractional uncertainty of approximately…
Tricationic protactinium monofluoride ($^{229}$PaF$^{3+}$) has been proposed as a candidate for probing physics beyond the Standard Model of particle physics. Since studies with $^{229}$PaF$^{3+}$ require significant experimental advances,…
A key advantage of quantum metrology is the ability to surpass the standard quantum limit~(SQL) for measurement precision through the use of non-classical states. However, there is typically little to no improvement in precision with the…
The generation of vortex matter waves carrying quantized orbital angular momentum is challenging and relies heavily on the material nanofabrication methods due to their extremely small de-Broglie wavelengths. Here, we introduce an…
We report relativistic many-body calculations of the interelectronic-interaction correction to the Land\'{e} $g$-factor of the $2s_{1/2}$, $2p_{1/2}$, $2p_{3/2}$, and $3s_{1/2}$ states in lithium-like ions with nuclear charge $Z = 4-20$.…
The open inner-shell electronic structure of lanthanides with large magnetic moments gives rise to a rich spectrum of transitions available for laser cooling, trapping, and coherent control. Despite this, the large number of ultraviolet…
Silver is a key tracer of the weak r-process in late-type stars. However, when the assumption of local thermodynamic equilibrium (LTE) needs to be relaxed, accurate abundance determinations become even more sensitive to complete sets of…
Motivated by the needs of atomic tritium sources for neutrino mass experiments and Doppler-free two-photon 1S-2S spectroscopy in atomic deuterium and tritium, we present calculations of energy-dependent elastic scattering cross sections of…
A calculation of the QED vacuum polarization potential in the Coulomb field of a pointlike nucleus was presented in an earlier publication by the author and his collaborators. Corrections up to order $\alpha^2 (Z\alpha)^7$ were evaluated,…
We present a machine learning model for predicting the electric dipole moment of diatomic molecules using only the atomic properties of the constituent atoms. Our model can screen the entire periodic table and identify the molecules with…