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A delay-programmable two-color femtosecond source for multiphoton ionization studies based on chirped-seed NOPA

Atomic Physics 2026-05-05 v1 Optics Quantum Physics

Abstract

We demonstrate a delay-programmable two-color femtosecond source based on a chirped-seed noncollinear optical parametric amplifier. Introducing controlled dispersion into the seed enables spectral selection through pump-seed delay, allowing flexible generation of two independently tunable pulse components with adjustable relative timing at high repetition rate. The temporal and spectral properties are characterized using nonlinear optical cross-correlation and dispersion-scan measurements. As a benchmark application, the source is employed in a COLTRIMS-based multiphoton ionization experiment on trapped Li atoms, revealing delay-dependent ionization pathways and demonstrating its suitability for bichromatic ultrafast spectroscopy.

Keywords

Cite

@article{arxiv.2605.02749,
  title  = {A delay-programmable two-color femtosecond source for multiphoton ionization studies based on chirped-seed NOPA},
  author = {Kyle Foster and Shruti Majumdar and Mason Toombs and Harshit Agarwal and Daniel Fischer},
  journal= {arXiv preprint arXiv:2605.02749},
  year   = {2026}
}