English

Strong-field ionization and AC-Stark shifted Rydberg states in OCS

Atomic Physics 2023-04-26 v1

Abstract

We present theoretical results for intensity-dependent above-threshold ionization (ATI) spectra from oriented OCS molecules probed by intense femtosecond laser pulses with wavelengths of 800 and 400 nm. The calculations were performed using the time-dependent Schroodinger equation within the single-active-electron approximation and including multielectron polarization effects. The results are in qualitative agreement with experimental data [Yu et al., J. Phys. B: At. Mol. Opt. Phys. 50, 235602 (2017)]. In particular, characteristic features in the ATI spectra which correspond to resonant multiphoton ionization via highly-excited Rydberg states are captured by the theory.

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Cite

@article{arxiv.2212.04664,
  title  = {Strong-field ionization and AC-Stark shifted Rydberg states in OCS},
  author = {Mahmoud Abu-samha and Lars Bojer Madsen},
  journal= {arXiv preprint arXiv:2212.04664},
  year   = {2023}
}

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3 figures