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Stripes in heterovalent metal-doped cuprates

General Physics 2021-08-06 v9

Abstract

Doping La2CuO4La_2CuO_{4} with alkaline-earth, Ae=Sr,BaAe= Sr,Ba generates holes in La2yxLnyAexCuO4La_{2-y-x}Ln_yAe_xCuO_{4} (Ln=Ln = Nd,EuNd,Eu). A small fraction of the holes, pˇ\check{p} \le 0.020.02, suppresses 3D-AFM. The rest resides as double holes at OO atoms in the CuO2CuO_2 planes. The superlattice, formed by the OO atoms, gives rise to both charge order stripes and magnetization stripes with incommensurability qc,m(x)xpˇq_{c,m}(x) \propto \sqrt{x-\check{p}} for AeAe doping x<x^x < \hat{x}, but constant qcq_c beyond. Antiparallel orientation of magnetic moments m(O)\mathbf{m}(O) yields a natural explanation for the coupling of qm(x)=12qc(x)q_m(x) = \frac{1}{2} q_c(x). Doping Nd2CuO4Nd_2CuO_{4} with CeCe generates electrons that reside pairwise in copper atoms. This accounts for the different properties of nn-doped compounds. When nn-doped, qc(x)xq_c(x) \propto \sqrt{x}. Above a threshold temperature TT', electron-hole pairs are thermally generated, but then separate to reside pairwise at CuCu and OO atoms. This breaks the locking of the incommensurability of charge order and magnetization stripes, qm(x)12qc(x)q_m(x) \ne \frac{1}{2} q_c(x).

Keywords

Cite

@article{arxiv.2002.12116,
  title  = {Stripes in heterovalent metal-doped cuprates},
  author = {Manfred Bucher},
  journal= {arXiv preprint arXiv:2002.12116},
  year   = {2021}
}

Comments

29 pages, 4 figures, 3 tables, 2 appendices. Change from the previous version: Minor corrections in Figs. 1 and 2