The non-relativistic spin-momentum locking in altermagnets gives rise to a time-reversal-odd spin Hall effect, known as the altermagnetic spin-splitting effect (ASSE). Although ASSE was first reported in RuO2, subsequent experiments have yielded inconsistent results, leaving its spin-transport mechanism unclear. Here, we systematically investigate how strain, crystal orientation, and the Hubbard U parameter influence the magnetic ground state and spin Hall response of RuO2. Guided by recent experimental observations, we find that U is likely smaller than the value required to induce intrinsic magnetism, suggesting that bulk RuO2 and (001)/(101) RuO2 thin films grown on TiO2 are nonmagnetic in the absence of extrinsic effects. In contrast, (100) and (110) films exhibit strain-induced altermagnetic spin splitting, leading to a strong ASSE even without Hubbard U corrections. These results reconcile previous experimental discrepancies and provide design guidelines for RuO2-based spintronic devices.
@article{arxiv.2602.11602,
title = {Strain-Driven Altermagnetic Spin Splitting Effect in RuO$_2$},
author = {Seungjun Lee and Seung Gyo Jeong and Jian-Ping Wang and Bharat Jalan and Tony Low},
journal= {arXiv preprint arXiv:2602.11602},
year = {2026}
}