English

Stability of the spiral spin liquid in MnSc$_2$S$_4$

Strongly Correlated Electrons 2018-09-05 v2 Materials Science

Abstract

We investigate the stability of the spiral spin liquid phase in MnSc2_2S4_4 against thermal and quantum fluctuations as well as against perturbing effects of longer-range interactions. Employing ab initioab~initio density functional theory (DFT) calculations we propose a realistic Hamiltonian for MnSc2_2S4_4, featuring second (J2J_2) and third (J3)(J_3) neighbor Heisenberg interactions on the diamond lattice that are considerably larger than previously assumed. We argue that the combination of strong J2J_2 and J3J_3 couplings reproduces the correct magnetic Bragg peak position measured experimentally. Calculating the spin-structure factor within the pseudofermion functional-renormalization group technique we find that close to the magnetic phase transition the sizable J3J_3 couplings induce a strong spiral selection effect, in agreement with experiments. With increasing temperature the spiral selection becomes weaker such that in a window around three to five times the ordering temperature an approximate spiral spin liquid is realized in MnSc2_2S4_4.

Keywords

Cite

@article{arxiv.1802.00357,
  title  = {Stability of the spiral spin liquid in MnSc$_2$S$_4$},
  author = {Yasir Iqbal and Tobias Müller and Harald O. Jeschke and Ronny Thomale and Johannes Reuther},
  journal= {arXiv preprint arXiv:1802.00357},
  year   = {2018}
}

Comments

11 pages, 10 figures, 1 table. Published version