Spin-reorientation as a switch for electronic topology in van der Waals ferromagnets
Abstract
The interplay between spin reorientation and topological electronic structure in two-dimensional (2D) van der Waals (vdW) ferromagnets is central to understanding how magnetic anisotropy shapes charge transport. Although spin-reorientation transitions (SRTs) are common in 2D metallic ferromagnets, their impact on electronic-topology-driven thermodynamic and transport properties remains largely unexplored. Here we investigate this issue in FeGeTe (F4GT), a room-temperature quasi-2D vdW ferromagnet, using temperature-dependent magnetization, specific heat, magnetotransport, and thermoelectric measurements. Magnetization and specific heat establish a reorientation of the magnetic easy axis near ~K, in addition to ferromagnetic ordering at ~K. Across the SRT, the Seebeck coefficient and anisotropic magnetoresistance show clear anomalies, indicating Fermi-surface reconstruction. The magnetoresistance exhibits a two-step field dependence: a low-field enhancement near the SRT associated with scattering from canted spins and evolving domains, followed by a higher-field negative response as spin fluctuations are suppressed. The simultaneous sign change of the ordinary Hall coefficient and the sharp anomaly in the anomalous Hall resistivity further point to a temperature-driven modification of the underlying band topology. Analysis of the anomalous Hall conductivity and the scaling of shows that the Berry-curvature-driven anomalous Hall response below is strongly modified above the transition. Our results identify spin reorientation as an internal control parameter for switching between distinct topological transport regimes in a 2D vdW ferromagnet, providing a symmetry-controlled route to engineer spin-polarized electronic states and domain-texture-driven functionalities.
Keywords
Cite
@article{arxiv.2603.20457,
title = {Spin-reorientation as a switch for electronic topology in van der Waals ferromagnets},
author = {Satyabrata Bera and Sudipta Chatterjee and Suman Kalyan Pradhan and Subhadip Pradhan and Arnab Bera and Sk Kalimuddin and Ashis K. Nandy and Mintu Mondal},
journal= {arXiv preprint arXiv:2603.20457},
year = {2026}
}