English

Spin-polaron fingerprints in the optical conductivity of iridates

Strongly Correlated Electrons 2026-04-16 v2

Abstract

As a consequence of their spin-orbit entangled ground state, many 5d55d^{5} iridate materials display a peculiar double peak structure in optical transport quantities, such as absorption and conductivity. Their common interpretation is based on the presence of Hubbard subbands in the half-filled jeff=1/2j_{\mathrm{eff}}=1/2 manifold. Herein, we challenge this picture, proposing a scenario based on the presence of spin-polaron (SP) quasiparticles, and assigning a dominant SP character to the first peak. We illustrate it by taking the materials Ba2_2IrO4_4 and Sr2_2IrO4_4 as paradigmatic examples, which we investigate within the dynamical mean-field theory and the self-consistent Born approximation. Both theories reproduce nontrivial features revealed by angle-resolved photoemission spectroscopy and optical transport measurements, supporting our interpretation. In the case of Sr2_2IrO4_4, we show how the SP scenario survives in the low-doped regime. Similar optical transport fingerprints are expected to be found in the wider class of 5d55d^5 iridates and more generally in strongly correlated antiferromagnetic regimes, such as those found in cuprates.

Keywords

Cite

@article{arxiv.2509.20337,
  title  = {Spin-polaron fingerprints in the optical conductivity of iridates},
  author = {Francesco Cassol and Léo Gaspard and Cyril Martins and Michele Casula and Benjamin Lenz},
  journal= {arXiv preprint arXiv:2509.20337},
  year   = {2026}
}

Comments

15 pages, 10 figures