English

Spin-density wave and superconductivity in La$_4$Ni$_3$O$_{10}$ under ambient pressure

Superconductivity 2025-05-12 v1

Abstract

We investigate the spin-density wave (SDW) behavior and the potential for superconductivity (SC) in La4_4Ni3_3O10_{10} under ambient pressure using a multi-orbital random-phase approximation (RPA). Starting with a twelve-orbital tight-binding model derived from density functional theory (DFT) calculations, we explore the influence of Hubbard interactions on SDW formation. Our analysis reveals a stripe-like SDW characterized by an incommensurate wave vector, Q(±0.7π,0)Q\approx(\pm 0.7\pi,0), suggesting a possible density wave instability in agreement with recent experiments. This configuration is driven by nesting of outer-layer Ni dz2d_{z^2} orbitals and exhibits interlayer antiferromagnetic ordering between the top and bottom NiO layers, with the middle layer serving as a node. We demonstrate that the Hund's coupling JHJ_H is the primary driver of the observed SDW. While superconductivity is absent in the undoped system under ambient pressure, it becomes attainable with appropriate hole doping (δ=0.4\delta=-0.4), resulting in a SC gap structure similar to the high-pressure phase. Our study identifies the specific conditions for realizing the ambient pressure stripe density wave: JH>0.16UJ_H>0.16U. Additionally, when doping leads to sufficient nesting at (0,0), the system's magnetic fluctuations transition into a stable Neel-type antiferromagnetic state, analogous to the high-pressure case.

Keywords

Cite

@article{arxiv.2411.12349,
  title  = {Spin-density wave and superconductivity in La$_4$Ni$_3$O$_{10}$ under ambient pressure},
  author = {Ming Zhang and Hongyi Sun and Yu-Bo Liu and Qihang Liu and Wei-Qiang Chen and Fan Yang},
  journal= {arXiv preprint arXiv:2411.12349},
  year   = {2025}
}

Comments

6 pages, 7 figures