English

Anisotropic Spin Stripe Domains in Bilayer La$_3$Ni$_2$O$_7$

Superconductivity 2025-09-04 v2 Strongly Correlated Electrons

Abstract

The discovery of superconductivity in La3_3Ni2_2O7_7 under pressure has motivated the investigation of a parent spin density wave (SDW) state, which could provide the underlying pairing interaction. Here, we employ resonant soft x-ray scattering and polarimetry on thin films of bilayer La3_3Ni2_2O7_7 to determine that the magnetic structure of the SDW forms unidirectional diagonal spin stripes with moments lying within the NiO2_2 plane and perpendicular to QSDW\mathbf{Q}_{SDW}, but without evidence of the strong charge disproportionation typically associated with other nickelates. These stripes form anisotropic domains with shorter correlation lengths perpendicular versus parallel to QSDW\mathbf{Q}_{SDW}, revealing nanoscale rotational and translational symmetry breaking analogous to the cuprate and Fe-based superconductors, with possible Bloch-like antiferromagnetic domain walls separating orthogonal domains.

Keywords

Cite

@article{arxiv.2409.03210,
  title  = {Anisotropic Spin Stripe Domains in Bilayer La$_3$Ni$_2$O$_7$},
  author = {N. K Gupta and R. Gong and Y. Wu and M. Kang and C. T. Parzyck and B. Z. Gregory and N. Costa and R. Sutarto and S. Sarker and A. Singer and D. G. Schlom and K. M. Shen and D. G. Hawthorn},
  journal= {arXiv preprint arXiv:2409.03210},
  year   = {2025}
}

Comments

18 pages, 5 figures; replaced with published version. Supplementary information available at https://doi.org/10.1038/s41467-025-61653-w