English

Self-diffusion in binary blends of cyclic and linear polymers

Soft Condensed Matter 2022-03-21 v2 Materials Science

Abstract

A lattice model is used to estimate the self-diffusivity of entangled cyclic and linear polymers in blends of varying compositions. To interpret simulation results, we suggest a minimal model based on the physical idea that constraints imposed on a cyclic polymer by infiltrating linear chains have to be released, before it can diffuse beyond a radius of gyration. Both, the simulation, and recently reported experimental data on entangled DNA solutions support the simple model over a wide range of blend compositions, concentrations, and molecular weights.

Keywords

Cite

@article{arxiv.0801.3474,
  title  = {Self-diffusion in binary blends of cyclic and linear polymers},
  author = {Sachin Shanbhag},
  journal= {arXiv preprint arXiv:0801.3474},
  year   = {2022}
}

Comments

10 pages, 2 figures

R2 v1 2026-06-21T10:05:26.909Z