English

Resonant inelastic scattering spectra at the Ir $L$-edge in Na$_2$IrO$_3$

Strongly Correlated Electrons 2016-09-27 v1

Abstract

We analyze resonant x-ray scattering (RIXS) spectra in Na2_2IrO3_3 on the basis of the itinerant electron picture. Employing a multi-orbital tight-binding model on a honeycomb lattice, we find that the zigzag magnetic order is the most stable with sizable energy gap in the one-electron band within the Hartree-Fock approximation. We derive the RIXS spectra, which are connected to the generalized density-density correlation function. We calculate the spectra as a function of excitation energy ω\omega, within the random phase approximation. The spectra consist of the peaks with ω\omega <20<20 meV, and of the peaks with 0.4<ω<0.80.4<\omega<0.8 eV. The former peaks are composed of four bound states in the density-density correlation function, and may be identified as the magnetic excitations, while the latter peaks are composed of sixteen bound states below the energy continuum of individual electron-hole pair excitations, and may be identified as the excitonic excitations. The calculated spectra agree qualitatively with the recent RIXS experiment.

Keywords

Cite

@article{arxiv.1606.08006,
  title  = {Resonant inelastic scattering spectra at the Ir $L$-edge in Na$_2$IrO$_3$},
  author = {Jun-ichi Igarashi and Tatsuya Nagao},
  journal= {arXiv preprint arXiv:1606.08006},
  year   = {2016}
}

Comments

7 pages, 5 figures