English

Reduced thermal conductivity in molecular forests

Mesoscale and Nanoscale Physics 2021-01-15 v1 Materials Science Soft Condensed Matter

Abstract

Heat propagation in quasi-one dimensional materials (Q1DMs) often appears paradoxical. While an isolated Q1DM, such as a nanowire, carbon nanotube, or polymer, can exhibit a high thermal conductivity \k{appa}, forests of the same materials show a reduction in \k{appa}. Here, the complex structures of these assemblies have hindered the emergence of a clear molecular picture of this intriguing phenomenon. We combine multiscale (coarse-grained) simulation with the concepts known from polymer physics and thermal transport to unveil a generic (microscopic) picture of \k{appa} reduction in molecular forests. We show that a delicate balance between the bond orientations, the persistence length of the Q1DM and the flexural vibrations govern the knock-down of \k{appa}.

Keywords

Cite

@article{arxiv.2005.10685,
  title  = {Reduced thermal conductivity in molecular forests},
  author = {Aashish Bhardwaj and A. Srikantha Phani and Alireza Nojeh and Debashish Mukherji},
  journal= {arXiv preprint arXiv:2005.10685},
  year   = {2021}
}
R2 v1 2026-06-23T15:43:05.386Z