English

Questioning the relationship between the $\chi$4 susceptibility and the dynamical correlation length in a glass former

Soft Condensed Matter 2015-09-11 v3 Statistical Mechanics

Abstract

Clusters of fast and slow correlated particles, identified as dynamical heterogeneities (DHs), con-stitute a central aspect of glassy dynamics. A key ingredient of the glass transition scenario is asignificant increase of the cluster size ξ\xi4 as the transition is approached. In need of easy-to-computetools to measure ξ\xi4 , the dynamical susceptibility χ\chi4 was introduced recently, and used in various ex-perimental works to probe DHs. Here, we investigate DHs in dense microgel suspensions using imagecorrelation analysis, and compute both χ\chi4 and the four-point correlation function G4 . The spatialdecrease of G4 provides a direct access to ξ\xi4 , which is found to grow significantly with increasingvolume fraction. However, this increase is not captured by χ\chi4 . We show that the assumptions thatvalidate the connection between χ\chi4 and ξ\xi4 are not fulfilled in our experiments.

Keywords

Cite

@article{arxiv.1412.8130,
  title  = {Questioning the relationship between the $\chi$4 susceptibility and the dynamical correlation length in a glass former},
  author = {Rémy Colin and Ahmed Alsayed and Cyprien Gay and Bérengère Abou},
  journal= {arXiv preprint arXiv:1412.8130},
  year   = {2015}
}

Comments

The present version was accepted for publication in Soft Matter (http://pubs.rsc.org/en/journals/journalissues/sm)