The intermediate-valent polymorphs α- and β-YbAlB4 exhibit quantum criticality and other novel properties not usually associated with intermediate valence. Iron doping induces quantum criticality in α-YbAlB4 and magnetic order in both compounds. We report results of muon spin relaxation (μSR) experiments in the intermediate-valent alloys α-YbAl1−xFexB4, x=0.014 and 0.25. For x=0.014 we find no evidence for magnetic order down to 25 mK\@. The dynamic muon spin relaxation rate λd exhibits a power-law temperature dependence λd∝T−a, a=0.40(4), in the temperature range 100 mK--2 K, in disagreement with predictions by theories of antiferromagnetic (AFM) or valence quantum critical behavior. For x=0.25, where AFM order develops in the temperature range 7.5--10 K, where we find coexistence of meso- or macroscopically segregated paramagnetic and AFM phases, with considerable disorder in the latter down to 2 K.
@article{arxiv.1605.07993,
title = {Quantum Criticality and Inhomogeneous Magnetic Order in Fe-doped alpha-YbAlB4},
author = {D. E. MacLaughlin and K. Kuga and Lei Shu and O. O. Bernal and P. -C. Ho and S. Nakatsuji and K. Huang and Z. F. Ding and C. Tan and Jian Zhang},
journal= {arXiv preprint arXiv:1605.07993},
year = {2016}
}
Comments
9 pages, 10 figures, to be published in Phys. Rev. B