English

Anomalous quantum-critical spin dynamics in YFe2Al10

Strongly Correlated Electrons 2018-04-11 v2

Abstract

We report results of a muon spin relaxation (μ\muSR) study of YFe2_2Al10_{10}, a quasi-2D nearly-ferromagnetic metal in which unconventional quantum critical behavior is observed. No static Fe2+^{2+} magnetism, with or without long-range order, is found down to 19~mK\@. The dynamic muon spin relaxation rate~λ\lambda exhibits power-law divergences in temperature and magnetic field, the latter for fields that are too weak to affect the electronic spin dynamics directly. We attribute this to the proportionality of λ(ωμ,T)\lambda(\omega_\mu,T) to the dynamic structure factor~S(ωμ,T)S(\omega_\mu,T), where ωμ105\omega_\mu \approx 10^5--107 s110^7~\mathrm{s}^{-1} is the muon Zeeman frequency. These results suggest critical divergences of S(ωμ,T)S(\omega_\mu,T) in both temperature and frequency. Power-law scaling and a 2D dissipative quantum XY (2D-DQXY) model both yield forms for S(ω,T)S(\omega,T) that agree with neutron scattering data (ω1012 s1\omega \approx 10^{12}~\mathrm{s}^{-1}). Extrapolation to μ\muSR frequencies agrees semi-quantitatively with the observed temperature dependence of λ(ωμ,T)\lambda(\omega_\mu,T), but predicts frequency independence for ωμT\omega_\mu \ll T in extreme disagreement with experiment. We conclude that the quantum critical spin dynamics of YFe2_2Al10_{10} are not well understood at low frequencies.

Keywords

Cite

@article{arxiv.1801.03659,
  title  = {Anomalous quantum-critical spin dynamics in YFe2Al10},
  author = {Kevin Huang and Cheng Tan and Jian Zhang and Zhaofeng Ding and D. E. MacLaughlin and O. O. Bernal and P. -C. Ho and C. Baines and Liusuo Wu and M. C. Aronson and Lei Shu},
  journal= {arXiv preprint arXiv:1801.03659},
  year   = {2018}
}

Comments

5 figures

R2 v1 2026-06-22T23:42:21.368Z