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Pressure-Induced Metallization in Iron-Based Ladder Compounds Ba$_{1-x}$Cs$_x$Fe$_2$Se$_3$

Strongly Correlated Electrons 2017-02-01 v1

Abstract

Electrical resistivity measurements have been performed on the iron-based ladder compounds Ba1x_{1-x}Csx_xFe2_2Se3_3 (xx = 0, 0.25, 0.65, and 1) under high pressure. A cubic anvil press was used up to 8.0 GPa, whereas further higher pressure was applied using a diamond anvil cell up to 30.0 GPa. Metallic behavior of the electrical conductivity was confirmed in the xx = 0.25 and 0.65 samples for pressures greater than 11.3 and 14.4 GPa, respectively, with the low-temperature logT\log T upturn being consistent with weak localization of 2D electrons due to random potential. At pressures higher than 23.8 GPa, three-dimensional Fermi-liquid-like behavior was observed in the latter sample. No metallic conductivity was observed in the parent compounds BaFe2_2Se3_3 (xx = 0) up to 30.0 GPa and CsFe2_2Se3_3 (xx = 1) up to 17.0 GPa. The present results indicate that the origins of the insulating ground states in the parent and intermediate compounds are intrinsically different; the former is a Mott insulator, whereas the latter is an Anderson insulator owing to the random substitution of Cs for Ba.

Keywords

Cite

@article{arxiv.1612.05394,
  title  = {Pressure-Induced Metallization in Iron-Based Ladder Compounds Ba$_{1-x}$Cs$_x$Fe$_2$Se$_3$},
  author = {Takafumi Hawai and Chizuru Kawashima and Kenya Ohgushi and Kazuyuki Matsubayashi and Yusuke Nambu and Yoshiya Uwatoko and Taku J. Sato and Hiroki Takahashi},
  journal= {arXiv preprint arXiv:1612.05394},
  year   = {2017}
}

Comments

5 pages, 3 figures