English

Potassium self-diffusion in a K-rich single-crystal alkali feldspar

Materials Science 2017-01-12 v1

Abstract

The paper reports potassium diffusion measurements performed on gem-quality single-crystal alkali feldspar in the temperature range from 11691169 to 1021\mboxK1021 \, \mbox{K}. Natural sanidine from Volkesfeld, Germany was implanted with \mbox43\mboxK\mbox{}^{43}\mbox{K} at the ISOLDE/CERN radioactive ion-beam facility normal to the (001) crystallographic plane. Diffusion coefficients are well described by the Arrhenius equation with an activation energy of 2.4\mboxeV2.4 \, \mbox{eV} and a pre-exponential factor of 5×106\mboxm2/\mboxs5\times10^{-6} \, \mbox{m}^{2}/\mbox{s}, which is more than three orders of magnitude lower than the \mbox22\mboxNa\mbox{}^{22}\mbox{Na} diffusivity in the same feldspar and the same crystallographic direction. State-of-the-art considerations including ionic conductivity data on the same crystal and Monte Carlo simulations of diffusion in random binary alloy structures point to a correlated motion of K and Na through the interstitialcy mechanism.

Keywords

Cite

@article{arxiv.1701.02884,
  title  = {Potassium self-diffusion in a K-rich single-crystal alkali feldspar},
  author = {Fabian Hergemöller and Matthias Wegner and Manfred Deicher and Herbert Wolf and Florian Brenner and Herbert Hutter and Rainer Abart and Nicolaas A. Stolwijk},
  journal= {arXiv preprint arXiv:1701.02884},
  year   = {2017}
}
R2 v1 2026-06-22T17:47:02.219Z