English

Pitfalls and solutions for perovskite transparent conductors

Materials Science 2021-08-11 v1 Strongly Correlated Electrons

Abstract

Transparent conductors-nearly an oxymoron-are in pressing demand, as ultra-thin-film technologies become ubiquitous commodities. As current solutions rely on non-abundant elements, perovskites such as SrVO3 and SrNbO3 have been suggested as next generation transparent conductors. Our ab-initio calculations and analytical insights show, however, that reducing the plasma frequency below the visible spectrum by strong electronic correlations-a recently proposed strategy-unavoidably comes at a price: an enhanced scattering and thus a substantial optical absorption above the plasma edge. As a way out of this dilemma we identify several perovskite transparent conductors, relying on hole doping, somewhat larger bandwidths and separations to other bands.

Keywords

Cite

@article{arxiv.2009.14000,
  title  = {Pitfalls and solutions for perovskite transparent conductors},
  author = {Liang Si and Josef Kaufmann and Jan M. Tomczak and Zhicheng Zhong and Karsten Held},
  journal= {arXiv preprint arXiv:2009.14000},
  year   = {2021}
}