We use spin dynamics simulations to determine the origin of the unusual correlated diffuse scattering, characterised by half-moon shapes bridging the magnetic Bragg peaks, observed in the polarised elastic neutron scattering from manganese tungstate, MnWO\textsubscript{4}. We first fit a Heisenberg Hamiltonian with twelve nearest-neighbour exchange interactions and single-ion anisotropy to the experimental ground-state magnon dispersion. We then show via spin dynamics simulations that our model Hamiltonian both reproduces the experimentally observed half-moon features and captures their persistence into the paramagnetic regime. Moreover, we identify the three-dimensional, competing antiferromagnetic interactions driving this behavior. Our work complements earlier studies of half-moon-shaped signatures in pyrochlore and triangular structures, by providing insight into their origin in a zigzag chain geometry with three-dimensional competing exchange interactions.
@article{arxiv.2503.23704,
title = {Paramagnetic half-moon shaped diffuse scattering arising from 3D magnetic frustration},
author = {Nelly Natsch and Tara N. Tošić and Jian-Rui Soh and Nicola A. Spaldin},
journal= {arXiv preprint arXiv:2503.23704},
year = {2025}
}