English

Oxygen vacancies in strained SrTiO$_{3}$ thin films: formation enthalpy and manipulation

Materials Science 2017-05-24 v1

Abstract

We report the enthalpy of oxygen vacancy formation in thin films of electron-doped SrTiO3_{3}, under different degrees of epitaxial stress. We demonstrate that both compressive and tensile strain decrease this energy at a very similar rate, and promote the formation of stable doubly ionized oxygen vacancies. Moreover, we also show that unintentional cationic vacancies introduced under typical growth conditions, produce a characteristic rotation pattern of TiO6_6 octahedra. The local concentration of oxygen vacancies can be modulated by an electric field with an AFM tip, changing not only the local electrical potential, but also producing a non-volatile mechanical response whose sign (up/down) can be reversed by the electric field.

Keywords

Cite

@article{arxiv.1704.05620,
  title  = {Oxygen vacancies in strained SrTiO$_{3}$ thin films: formation enthalpy and manipulation},
  author = {L. Iglesias and A. Sarantopoulos and C. Magen and F. Rivadulla},
  journal= {arXiv preprint arXiv:1704.05620},
  year   = {2017}
}

Comments

Physical Review B (accepted for publication)