Overlapping resonances in the control of intramolecular vibrational redistribution
Quantum Physics
2007-05-23 v1
Abstract
Coherent control of bound state processes via the interfering overlapping resonances scenario [Christopher et al., J. Chem. Phys. 123, 064313 (2006)] is developed to control intramolecular vibrational redistribution (IVR). The approach is applied to the flow of population between bonds in a model of chaotic OCS vibrational dynamics, showing the ability to significantly alter the extent and rate of IVR by varying quantum interference contributions.
Keywords
Cite
@article{arxiv.quant-ph/0703263,
title = {Overlapping resonances in the control of intramolecular vibrational redistribution},
author = {D. Gerbasi and A. S. Sanz and P. S. Christopher and M. Shapiro and P. Brumer},
journal= {arXiv preprint arXiv:quant-ph/0703263},
year = {2007}
}
Comments
10 pages, 7 figures