English

Order from disorder phenomena in BaCoS$_2$

Strongly Correlated Electrons 2023-02-24 v1

Abstract

At TN305 KT_N\simeq 305~\text{K} the layered insulator BaCoS2_2 transitions to a columnar antiferromagnet that signals non-negligible magnetic frustration despite the relatively high TNT_N, all the more surprising given its quasi two-dimensional structure. Here, we show by combining ab initio and model calculations that the magnetic transition is an order-from-disorder phenomenon, which not only drives the columnar C4C2C_4\to C_2 symmetry breaking, but also, and more importantly, the inter-layer coherence responsible for the finite N\'eel transition temperature. This uncommon ordering mechanism, actively contributed by orbital degrees of freedom, hints at an abundance of low energy excitations below and, especially, above TNT_N, not in disagreement with experimental evidences, and might as well emerge in other layered correlated compounds showing frustrated magnetism at low temperature.

Keywords

Cite

@article{arxiv.2302.12179,
  title  = {Order from disorder phenomena in BaCoS$_2$},
  author = {Benjamin Lenz and Michele Fabrizio and Michele Casula},
  journal= {arXiv preprint arXiv:2302.12179},
  year   = {2023}
}

Comments

12 pages, 6 figures

R2 v1 2026-06-28T08:48:09.205Z