English

Orbital-selective charge-density wave in TaTe$_4$

Strongly Correlated Electrons 2023-11-07 v1 Materials Science

Abstract

TaTe4_4, a metallic charge-density wave (CDW) material discovered decades ago, has attracted renewed attention due to its rich interesting properties such as pressure-induced superconductivity and candidate non-trivial topological phase. Here, using high-resolution angle-resolved photoemission spectroscopy and ab-initio calculation, we systematically investigate the electronic structure of TaTe4_4. At 26 K, we observe a CDW gap as large as 290 meV, which persists up to 500 K. The CDW-modulated band structure shows a complex reconstruction that closely correlates with the lattice distortion. Inside the CDW gap, there exist highly dispersive energy bands contributing to the remnant Fermi surface and metallic behavior in the CDW state. Interestingly, our ab-initio calculation reveals that the large CDW gap mainly opens in the electronic states with out-of-plane orbital components, while the in-gap metallic states originate from in-plane orbitals, suggesting an orbital texture that couples with the CDW order. Our results shed light on the interplay between electron, lattice, and orbital in quasi-one-dimensional CDW materials.

Keywords

Cite

@article{arxiv.2308.08246,
  title  = {Orbital-selective charge-density wave in TaTe$_4$},
  author = {R. Z. Xu and X. Du and J. S. Zhou and X. Gu and Q. Q. Zhang and Y. D. Li and W. X. Zhao and F. W. Zheng and M. Arita and K. Shimada and T. K. Kim and C. Cacho and Y. F. Guo and Z. K. Liu and Y. L. Chen and L. X. Yang},
  journal= {arXiv preprint arXiv:2308.08246},
  year   = {2023}
}

Comments

to appear in npj Quantum Materials

R2 v1 2026-06-28T11:56:51.235Z