English

On-Surface Structural and Electronic Properties of Spontaneously Formed Tb$_2$Pc$_3$ Single Molecule Magnets

Mesoscale and Nanoscale Physics 2018-08-10 v1

Abstract

The single molecule magnet (SMM) bis(phthalocyaninato)terbium (III) (TbPc2_2) has attracted steady research attention as an exemplar system for realizing molecule-based spin electronics. In this paper, we report on the spontaneous formation of Tb2_2Pc3_3 species from TbPc2_2 precursors via sublimation in ultrahigh vacuum (UHV) onto an Ag(111) surface. The molecules on the surface are inspected using combined scanning tunneling (STM) and non-contact atomic force microscopies (nc-AFM) at 5 Kelvin. Submolecular resolution and height dependent measurements supported by density functional theory (DFT) calculations unambiguously show the presence of both TbPc2_2 and Tb2_2Pc3_3 species. The synthesis of Tb2_2Pc3_3 species under UHV conditions is independently confirmed by chemical analysis. The high-resolution AFM imaging allows us to register the orientation of the topmost Pc ligand in both Tb2_2Pc3_3 and TbPc2_2 relative to the underlying Ag(111) surface. Measurements of the electronic structure reveal the selective appearance of a Kondo signature with temperature \sim 30K in the Tb2_2Pc3_3 species, localized to the Pc ligand lobes. We attribute the presence of the Kondo resonance on select Tb2_2Pc3_3 molecules to the orientation of internal molecular ligands. High-resolution AFM imaging identifies geometric distortions between Tb2_2Pc3_3 molecules with and without the Kondo effect, the result of the complex interplay between structural and electronic differences.

Keywords

Cite

@article{arxiv.1805.03913,
  title  = {On-Surface Structural and Electronic Properties of Spontaneously Formed Tb$_2$Pc$_3$ Single Molecule Magnets},
  author = {Jack Hellerstedt and Aleš Cahlík and Martin Švec and Bruno de la Torre and María Moro-Lagares and Barbora Papoušková and Giorgio Zoppellaro and Pingo Mutombo and Mario Ruben and Radek Zbořil and Pavel Jelinek},
  journal= {arXiv preprint arXiv:1805.03913},
  year   = {2018}
}

Comments

29 pages, 8 figures; additional supplementary information in /anc directory