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With recent advances in the areas of nanostructure fabrication and molecular spintronics the idea of using single molecule magnets as building blocks for the next generation electronic devices becomes viable. A particular example represents…

Mesoscale and Nanoscale Physics · Physics 2020-03-10 Ivan I. Vrubel , Anastasiia A. Pervishko , Heike Herper , Barbara Brena , Olle Eriksson , Dmitry Yudin

The spintronic properties of magnetic molecules have attracted significant scientific attention. Special emphasis has been placed on the qubit for quantum information processing. The single molecule magnet, bis(phthalocyaninato (Pc))…

We report manipulation of a Kondo resonance originated from the spin-electron interactions between a two-dimensional molecular assembly of TBrPP-Co molecules and a Cu(111) surface at 4.6 K using a low temperature scanning tunneling…

Materials Science · Physics 2015-06-25 Violeta Iancu , Aparna Deshpande , Saw-Wai Hla*

Complex magneto structural behaviour of rare rich intermetallic Tb$_3$Co is reported in this study. Below the 84K (T$_N$), it undergoes a first order magnetic transition 72K confirmed from specific heat and magnetization measurements.…

Materials Science · Physics 2019-08-23 Srikanta Goswami , P. D. Babu , R. Rawat

We investigate how different chemical environment influences magnetic properties of terbium(III) (Tb)-based single-molecule magnets (SMMs), using first-principles relativistic multireference methods. Recent experiments showed that Tb-based…

Chemical Physics · Physics 2020-07-01 Ryan Pederson , Aleksander L. Wysocki , Nicholas Mayhall , Kyungwha Park

Magnetization, AC susceptibility and $\mu$SR measurements have been performed in neutral phthalocyaninato lanthanide ([LnPc$_2]^0$) single molecule magnets in order to determine the low-energy levels structure and to compare the…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 F. Branzoli , P. Carretta , M. Filibian , M. J. Graf , S. Klyatskaya , M. Ruben , F. Coneri , P. Dhakal

We study Kondo physics of a spin-$\frac{1}{2}$ impurity in electronic matter with strong spin-orbit interaction, which can be realized by depositing magnetic adatoms on the surface of a three-dimensional topological insulator. We show that…

Strongly Correlated Electrons · Physics 2015-12-10 L. Isaev , G. Ortiz , I. Vekhter

A key to building functional devices on the basis of single molecule magnets in the framework of molecular electronics is the ability to deposit and study these molecules on a surface, because the structural, electronic and magnetic…

Mesoscale and Nanoscale Physics · Physics 2016-01-26 Judith Donner , Jan-Philipp Broschinski , Bastian Feldscher , Anja Stammler , Hartmut Bögge , Thorsten Glaser , Daniel Wegner

Individual magnetic molecules are promising building blocks for quantum technologies because of their chemical tunability, nanoscale dimensions, and ability to self-assemble into ordered arrays. However, harnessing their properties in…

Metalated phthalocyanines (Pc's) are robust and versatile molecular complexes, whose properties can be tuned by changing their functional groups and central metal atom. The electronic structure of magnesium Pc (MgPc) - structurally and…

Lanthanide-based single-ion magnetic molecules can have large magnetic hyperfine interactions as well as large magnetic anisotropy. Recent experimental studies reported tunability of these properties by changes of chemical environments or…

Materials Science · Physics 2019-10-29 Aleksander L. Wysocki , Kyungwha Park

The hybridization of magnetism and superconductivity has been an intriguing playground for correlated electron systems, hosting various novel physical phenomena. Usually, localized d- or f-electrons are central to magnetism. In this study,…

Magnetic topological materials are a class of compounds which can host massless electrons controlled by the magnetic order. One such compound is EuZn$_2$Sb$_2$, which has recently garnered interest due to its strong interplay between the Eu…

Strongly Correlated Electrons · Physics 2026-02-17 Yu Wei Soh , Hsiang Lee , Eugen Weschke , Shinichi Nishihaya , Mikhael T. Sayat , Masaki Uchida , Jian-Rui Soh

Magnetization versus field measurements were performed on single crystals of [(Pc)2TbIII0.02YIII0.98]^TBA+ and [(Pc)2DyIII0.02YIII0.98]^TBA+ (Pc: phthalocyaninato, TBA: tetrabutylammonium) at 0.04 K. The [(Pc)2TbIII] complex, the first…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 N. Ishikawa , M. Sugita , W. Wernsdorfer

Electron charging play key roles in physiochemical processes, whose intrinsic stabilization in single molecules is desirable for tailoring molecular functionality and developing molecular devices, but remains elusive on surfaces. Here, we…

Mesoscale and Nanoscale Physics · Physics 2025-03-11 Xin Liao , Rui-Jing Sun , Emi Minamitani , Lian-Zhi Yang , Tao Xie , Wen-Hao Zhang , Chaofei Liu , Svetlana Klyatskaya , Mario Ruben , Ying-Shuang Fu

Well-ordered organic molecular layers on oxide surfaces are key for organic electronics. Using a combination of scanning tunneling microscopy (STM) and non-contact atomic force microscopy (nc-AFM) we probe the structures of copper…

We report the structural and magnetic properties of a quantum magnet PbCuTeO5. The triclinic structure of PbCuTeO5 comprises of alternating layers (ab-planes), in which one layer is composed of S = 1/2 dimer chains and another layer is…

Strongly Correlated Electrons · Physics 2017-05-31 B. Koteswararao , S. P. Chilakalapudi , Aga Shahee , P. V. Srinivasarao , S. Srinath , A. V. Mahajan

We study the Kondo physics of a quantum magnetic impurity in two-dimensional topological superconductors (TSCs), either intrinsic or induced on the surface of a bulk topological insulator, using a numerical renormalization group technique.…

Superconductivity · Physics 2019-03-06 Rui Wang , W. Su , Jian-Xin Zhu , C. S. Ting , Hai Li , Changfeng Chen , Baigeng Wang , Xiaoqun Wang

Using a state-of-the art combination of density functional theory and impurity solver techniques we present a complete and parameter-free picture of the Kondo effect in the high-spin ($S=3/2$) coordination complex known as Manganese…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 D. Jacob , M. Soriano , J. J. Palacios

We report on the synthesis and magnetic properties of Mn12-based single molecular magnets (SMMs) with benzene and pentafluorobenzene carboxylate ligands. The changes in ligand structure are shown to have a decisive effect on magnetic…

Strongly Correlated Electrons · Physics 2011-11-08 V. S. Zagaynova , T. L. Makarova , N. G. Spitsina , D. W. Boukhvalov
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