English

Magnon interactions in the frustrated pyrochlore ferromagnet Yb$_2$Ti$_2$O$_7$

Strongly Correlated Electrons 2019-09-19 v1

Abstract

The frustrated rare-earth pyrochlore Yb2_2Ti2_2O7_7 is remarkable among magnetic materials: despite a ferromagnetically ordered ground state it exhibits a broad, nearly gapless, continuum of excitations. This broad continuum connects smoothly to the sharp one-magnon excitations expected, and indeed observed, at high magnetic fields, raising the question: how does this picture of sharp magnons break down as the field is lowered? In this paper, we consider the effects of magnon interactions in Yb2_2Ti2_2O7_7, showing that their inclusion greatly extends the reach of spin-wave theory. First, we show that magnon interactions shift the phase boundary between the (splayed) ferromagnet (SFM) and the antiferromagnetic Γ5\Gamma_5 phase so that Yb2_2Ti2_2O7_7 lies very close to it. Next, we show how the high-field limit connects to lower fields; this includes corrections to the critical fields for the [111][111] and [11ˉ0][1\bar{1}0] directions, bringing them closer to the observed experimental values, as well as accounting for the departures from linear spin wave theory that appear in [001][001] applied fields below 3 T [Thompson et al., Phys. Rev. Lett. 119, 057203 (2017)]. Turning to low-fields, though the extent of the experimentally observed broadening is not quite reproduced, we find a rough correspondence between non-linear spin-wave theory and inelastic neutron scattering data on both a single-crystal sample, as well as on a powder sample [Pe\c{c}anha-Antonio et al., Phys. Rev. B, 96, 214415 (2017)]. We conclude with an outlook on implications for future experimental and theoretical work on Yb2_2Ti2_2O7_7 and related materials, highlighting the importance of proximity to the splayed ferromagnet-Γ5\Gamma_5 phase boundary and its potential role in intrinsic or extrinsic explanations of the low-field physics of Yb2_2Ti2_2O7_7.

Keywords

Cite

@article{arxiv.1903.05098,
  title  = {Magnon interactions in the frustrated pyrochlore ferromagnet Yb$_2$Ti$_2$O$_7$},
  author = {Jeffrey G. Rau and Roderich Moessner and Paul A. McClarty},
  journal= {arXiv preprint arXiv:1903.05098},
  year   = {2019}
}

Comments

19 pages, 12 figures