English

Linewidths in excitonic absorption spectra of cuprous oxide

Materials Science 2016-02-17 v1 Mesoscale and Nanoscale Physics Quantum Physics

Abstract

We present a theoretical calculation of the absorption spectrum of cuprous oxide (Cu2O)\left(\mathrm{Cu_{2}O}\right) based on the general theory developed by Y. Toyozawa. An inclusion not only of acoustic phonons but also of optical phonons and of specific properties of the excitons in Cu2O\mathrm{Cu_{2}O} like the central-cell corrections for the 1S1S-exciton allows us to calculate the experimentally observed line widths in experiments by T. Kazimierczuk et al [Nature 514, 343, (2014)] within the same order of magnitude, which demonstrates a clear improvement in comparison to earlier work on this topic. We also discuss a variety of further effects, which explain the still observable discrepancy between theory and experiment but can hardly be included in theoretical calculations.

Keywords

Cite

@article{arxiv.1602.01813,
  title  = {Linewidths in excitonic absorption spectra of cuprous oxide},
  author = {Frank Schweiner and Jörg Main and Günter Wunner},
  journal= {arXiv preprint arXiv:1602.01813},
  year   = {2016}
}