English

Large electrocaloric strength in ferroelectric nematic liquid crystals with a tuneable operational temperature range

Soft Condensed Matter 2025-10-31 v1 Materials Science

Abstract

The electrocaloric (EC) effect offers a promising energy-efficient and clean cooling technology. We present the first direct measurements of EC temperature change in a new family of EC fluids, ferroelectric nematic liquid crystals (FNLCs), demonstrating in two such materials temperature jumps of ΔTj|{\Delta}T_j| ~ 0.2 K for field changes as low as ΔE{\Delta}E ~ 0.1 Vμm1V {\mu}m^{-1}. Indirect measurements of adiabatic temperature change ΔT|{\Delta}T| confirm that these direct measurements are an underestimate and that ΔE{\Delta}E = 2 Vμm1V {\mu}m^{-1} can induce up to ΔT|{\Delta}T| ~ 1.6 K, yielding EC strengths ΔT/ΔE|{\Delta}T/{\Delta}E| up to 100% higher than incumbent materials. For temperature spans of 5-10 K, we predict a coefficient of performance of ~21-40. We find ΔT|{\Delta}T| ~ 1 K for >100 FNLCs that collectively span all temperatures between 00{^\circ}C and 100100{^\circ}C. This, together with the new device concepts conceivable with fluid EC materials, offers huge potential for cooling applications.

Keywords

Cite

@article{arxiv.2510.26386,
  title  = {Large electrocaloric strength in ferroelectric nematic liquid crystals with a tuneable operational temperature range},
  author = {Diana I. Nikolova and Rachel Tuffin and Mengfan Guo and Neil D. Mathur and Xavier Moya and Peter Tipping and Richard J. Mandle and Helen F. Gleeson},
  journal= {arXiv preprint arXiv:2510.26386},
  year   = {2025}
}

Comments

13 pages, 6 figures. Submitted to Nature Energy