We report a neutron diffraction study of single-crystal CePtAl3 complemented by measurements of the specific heat under applied magnetic field. Below TN=3 K CePtAl3 develops incommensurate antiferromagnetic order with a single modulation vector k=(0.67600). Residual magnetic scattering intensity above TN and a broadening of the specific heat anomaly at TN may be consistently described in terms of a Gaussian distribution of transition temperatures with a standard deviation σ≈0.5K. The distribution of TN may be attributed to the observation of occupational and positional disorder between the Pt and Al sites. Measurements under magnetic field reveal unusual changes of the domain populations when the field is applied along the [010] direction consistent with a transition from cycloidal to amplitude modulated magnetic order around 2.5 T.
@article{arxiv.2106.08194,
title = {Incommensurate antiferromagnetic order in CePtAl$_3$},
author = {M. Stekiel and P. Cermak and C. Franz and W. Simeth and S. Weber and E. Ressouche and W. Schmidt and K. Nemkovski and H. Deng and A. Bauer and C. Pfleiderer and A. Schneidewind},
journal= {arXiv preprint arXiv:2106.08194},
year = {2023}
}
Comments
v1: Draft on CePtAl3 and CePdAl3. Later split into separate papers regarding each compound separately. v2: Before submission. Major reworks from v1. v3: Final. After peer review and proofs