English

Higher-order topological insulators in two-dimensional antiferromagnetic and altermagnetic chromium-based group-IV chalcogenides

Materials Science 2026-04-13 v1

Abstract

Based on first-principles calculations combined with theoretical analysis, we identify a family of monolayer chromium-based group-IV chalcogenides as a new class of two-dimensional (2D) magnetic higher-order topological insulators (HOTIs). Specifically, the CrCX3X_3 (X=X= S, Se, Te) and CrSiS3_3 monolayers are found to host conventional antiferromagnetic ground states with PT\mathcal{PT} symmetry, whereas the Janus compounds Cr2_2C2_2S3_3Se3_3 and Cr2_2Si2_2S3_3Se3_3 exhibit altermagnetic ground states. We demonstrate that all these monolayer magnetic materials realize 2D HOTI phases, in which the nontrivial topology is protected by lattice C3C_3 rotational symmetry and manifests as zero-dimensional corner states carrying quantized fractional charges. Moreover, upon inclusion of spin-orbit coupling, these systems remain in the HOTI phase and continue to host robust corner-localized states, confirming the stability of their higher-order topological nature. Our results reveal an intrinsic connection between higher-order topology and magnetic order in 2D antiferromagnetic and altermagnetic systems, identifying chromium-based group-IV chalcogenide monolayers as promising platforms for exploring higher-order topological phases and their potential relevance for future topological and spintronic applications.

Keywords

Cite

@article{arxiv.2604.08907,
  title  = {Higher-order topological insulators in two-dimensional antiferromagnetic and altermagnetic chromium-based group-IV chalcogenides},
  author = {Ruo-Yu Ning and Yong-Kun Wang and Shifeng Qian and Si Li and Wen-Li Yang},
  journal= {arXiv preprint arXiv:2604.08907},
  year   = {2026}
}

Comments

8 pages, 5 figures