English

Harmonic chain far from equilibrium: single-file diffusion, long-range order, and hyperuniformity

Statistical Mechanics 2024-10-02 v4 Soft Condensed Matter

Abstract

In one dimension, particles can not bypass each other. As a consequence, the mean-squared displacement (MSD) in equilibrium shows sub-diffusion MSD(t)t1/2{\rm MSD}(t)\sim t^{1/2}, instead of normal diffusion MSD(t)t{\rm MSD}(t)\sim t. This phenomenon is the so-called single-file diffusion. Here, we investigate how the above equilibrium behaviors are modified far from equilibrium. In particular, we want to uncover what kind of non-equilibrium driving force can suppress diffusion and achieve the long-range crystalline order in one dimension, which is prohibited by the Mermin-Wagner theorem in equilibrium. For that purpose, we investigate the harmonic chain driven by the following four types of driving forces that do not satisfy the detailed balance: (i) temporally correlated noise with the noise spectrum D(ω)ω2θD(\omega)\sim \omega^{-2\theta}, (ii) conserving noise, (iii) periodic driving force, and (iv) periodic deformations of particles. For the driving force (i) with θ>1/4\theta>-1/4, we observe MSD(t)t1/2+2θ{\rm MSD}(t)\sim t^{1/2+2\theta} for large tt. On the other hand, for the driving forces (i) with θ<1/4\theta<-1/4 and (ii)-(iv), MSD remains finite. As a consequence, the harmonic chain exhibits the crystalline order even in one dimension. Furthermore, the density fluctuations of the model are highly suppressed in a large scale in the crystal phase. This phenomenon is known as hyperuniformity. We discuss that hyperuniformity of the noise fluctuations themselves is the relevant mechanism to stabilize the long-range crystalline order in one dimension and yield hyperuniformity of the density fluctuations.

Keywords

Cite

@article{arxiv.2309.03155,
  title  = {Harmonic chain far from equilibrium: single-file diffusion, long-range order, and hyperuniformity},
  author = {Harukuni Ikeda},
  journal= {arXiv preprint arXiv:2309.03155},
  year   = {2024}
}

Comments

23 pages, 7figures

R2 v1 2026-06-28T12:14:29.382Z